Shell effects on fission barriers of metallic clusters: A systematic description

被引:6
|
作者
Vieira, A [1 ]
Fiolhais, C [1 ]
机构
[1] Univ Coimbra, Dept Fis, P-3000 Coimbra, Portugal
来源
PHYSICAL REVIEW B | 1998年 / 57卷 / 12期
关键词
D O I
10.1103/PhysRevB.57.7352
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We use the liquid drop model, with the stabilized jellium model, and the Strutinsky shell correction method [Nucl. Phys. A 95, 420 (1967); 122, 1 (1968)], with the two-center asymmetric deformed harmonic-oscillator potential, to evaluate fission barriers for three representative simple metal clusters (sodium, aluminum, and potassium). We obtain fission barrier heights as a function of size, charge, and mass asymmetry for all possible decay channels of doubly charged clusters with up to 30 atoms. We show how fragment deformations change the barrier height. For small sodium and potassium clusters we find good agreement of the fission barriers with molecular-dynamics calculations. The critical number (cluster size for which fission competes with evaporation) is correctly reproduced for doubly charged clusters of the three metals considered.
引用
收藏
页码:7352 / 7359
页数:8
相关论文
共 50 条
  • [41] First principles description of shell structure in metal clusters
    Kamimura, H
    Sugino, O
    FEW-BODY PROBLEMS IN PHYSICS '99, 2000, 12 : 15 - 24
  • [42] PATTERNS AND BARRIERS FOR FISSION OF CHARGED SMALL METAL-CLUSTERS - REPLY
    BARNETT, RN
    LANDMAN, U
    PHYSICAL REVIEW LETTERS, 1992, 69 (09) : 1472 - 1472
  • [43] PATTERNS AND BARRIERS FOR FISSION OF CHARGED SMALL METAL-CLUSTERS - COMMENT
    JENA, P
    KHANNA, SN
    YANNOULEAS, C
    PHYSICAL REVIEW LETTERS, 1992, 69 (09) : 1471 - 1472
  • [44] Similarities and differences in fission and evaporation of hot nuclei and hot metallic clusters
    Frobrich, P
    JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS, 1997, 23 (10) : 1439 - 1449
  • [45] Calculations of fission barriers with deformation-dependent attenuation of shell corrections
    Shvedov, L
    Blocki, J
    Wilczynski, J
    ACTA PHYSICA POLONICA B, 2002, 33 (01): : 439 - 444
  • [46] FISSION BARRIERS FOR CM ISOTOPES - WHAT IS NATURE OF N=152 SHELL
    BACK, BB
    HANSEN, O
    BRITT, HC
    GARRETT, JD
    PHYSICS LETTERS B, 1973, B 46 (02) : 183 - 185
  • [47] ESTIMATION OF TEMPERATURE EFFECTS ON FISSION-BARRIERS
    PI, M
    VINAS, X
    BARRANCO, M
    PHYSICAL REVIEW C, 1982, 26 (02): : 733 - 735
  • [48] SHELL CORRECTION STUDY OF FISSION OF DOUBLY-CHARGED SILVER CLUSTERS
    KOIZUMI, H
    SUGANO, S
    ISHII, Y
    ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1993, 28 (03): : 223 - 234
  • [49] DESCRIPTION OF METALLIC AND COVALENT CLUSTERS WITH ICOSAHEDRAL SYMMETRY - THE POLYTOPE MODEL
    MOSSERI, R
    SADOC, JF
    ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1989, 12 (1-4): : 89 - 92
  • [50] SIMPLIFIED SEMICLASSICAL THEORY FOR THE ELECTRONIC SHELL STRUCTURE OF METALLIC CLUSTERS
    STAMPFLI, P
    BENNEMANN, KH
    ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1992, 25 (01): : 87 - 94