Performance Evaluation of Aqueous Carbonation for Steelmaking Slag: Process Chemistry

被引:6
|
作者
Pan, Shu-Yuan [1 ]
Chiang, Pen-Chi [1 ]
Chen, Yi-Hung [2 ]
Chen, Chun-Da [3 ]
Lin, Hsun-Yu [3 ]
Chang, E-E [4 ]
机构
[1] Natl Taiwan Univ, Grad Inst Environm Engn, Taipei, Taiwan
[2] Natl Taipei Univ Technol, Dept Chem Engn & Biotechnol, Taipei, Taiwan
[3] China Steel Corp, New Mat Res & Dev Dept, Energy Dev & Applicat Sect, Kaohsiung, Taiwan
[4] Taipei Med Univ, Dept Biochem, Taipei, Taiwan
来源
GHGT-11 | 2013年 / 37卷
关键词
CO2; sequestration; thermogravimetric analysis; quantitative X-ray diffraction; Rietveld method; rotating packed bed; calcite; CO2; ASH;
D O I
10.1016/j.egypro.2013.05.091
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Accelerated carbonation of BOF slag in an RPB is a viable method for CO2 capture due to its high mass transfer rate. However, the process chemistry of carbonation of BOF slag is not well-determined due to their complex compositions. In this investigation, the quantitative X-ray diffraction was utilized to determine the mechanism of carbonation reaction in an RPB. Rietveld refinement, which aims to minimize the difference between the experimental and refined XRD patterns by a least-square procedure, is performed to quantify the crystallized mineral. In addition, changes of physico-chemical properties of BOF slags before and after carbonation were evaluated. (C) 2013 The Authors. Published by Elsevier Ltd.
引用
收藏
页码:115 / 121
页数:7
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