Influence of Li2O-B2O3-SiO2 glass on the sintering behavior and microwave dielectric properties of BaO-0.15ZnO-4TiO2 ceramics

被引:22
|
作者
Duan, Shuxin [1 ]
Li, Enzhu [1 ]
Chen, Hetuo [1 ]
Tang, Bin [1 ]
Yuan, Ying [1 ]
Zhang, Shuren [1 ]
机构
[1] Univ Elect Sci & Technol China, Sch Microelect & Solid State Elect, Chengdu 610054, Peoples R China
基金
中国国家自然科学基金; 高等学校博士学科点专项科研基金;
关键词
BaO-0.15ZnO-4TiO(2); LTCC; Li2O-B2O3-SiO2 (LBS); Microwave dielectric ceramics; HIGH-PERMITTIVITY; SYSTEM;
D O I
10.1016/j.ceramint.2016.01.174
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
This paper reports the investigation of the performance of Li2O-B2O3-SiO2 (LBS) glass as a sintering aid to lower the sintering temperature of BaO-0.15ZnO-4TiO(2) (BZT) ceramics, as well as the detailed study on the sintering behavior, phase evolution, microstructure and microwave dielectric properties of the resulting BZT ceramics. The addition of LBS glass significantly lowers the sintering temperature of the BZT ceramics from 1150 degrees C to 875-925 degrees C. Small amount of LBS glass promotes the densification of BZT ceramic and improves the dielectric properties. However, excessive LBS addition leads to the precipitation of glass phase and growth of abnormal grain, deteriorating the dielectric properties of the BZT ceramic. The BZT ceramic with 5 wt% LBS addition sintered at 900 degrees C shows excellent microwave dielectric properties: epsilon(r) = 27.88, Q x f = 14,795 GHz. (C) 2016 Elsevier Ltd and Techna Group S.r.l. All rights reserved.
引用
收藏
页码:7943 / 7949
页数:7
相关论文
共 50 条
  • [31] Low-fire processing of microwave BaTi4O9 dielectric with BaO-Li2O-B2O3-SiO2-ZnO glass
    Su, Yu-Sheng
    Jean, Jau-Ho
    [J]. Japanese Journal of Applied Physics, 2008, 47 (9 PART 1): : 7254 - 7256
  • [32] DIELECTRIC BEHAVIOR OF GLASSES AND GLASS-CERAMICS IN THE SYSTEM BAO-PBO-TIO2-B2O3-SIO2
    MANDAL, RK
    PRASAD, CD
    PARKASH, O
    KUMAR, D
    [J]. BULLETIN OF MATERIALS SCIENCE, 1987, 9 (04) : 255 - 262
  • [33] Influence of B2O3 on sintering behavior and the dielectric properties of Li2MgSiO4 ceramics
    Agathopoulos, Simeon
    [J]. JOURNAL OF THE CERAMIC SOCIETY OF JAPAN, 2012, 120 (1402) : 233 - 237
  • [34] Microwave dielectric properties and microstructures of BaO modified CaO-Li2O-Sm2O3-TiO2 ceramics
    Chen, HL
    Huang, CL
    Li, JL
    [J]. JOURNAL OF MATERIALS SCIENCE LETTERS, 2000, 19 (24) : 2197 - 2199
  • [35] Low-Temperature Sintering and Microwave Dielectric Properties of Li2O-3ZnO-5TiO2 Ceramics Doped with B2O3
    Liu, J.
    Zhu, J.
    Zeng, Y.
    [J]. JOURNAL OF CERAMIC SCIENCE AND TECHNOLOGY, 2019, 10 (02):
  • [36] Preparation and Properties of Li2Zn3Ti4O12-Based Ceramics with a Sintering Aid in the Li2O-B2O3-SiO2 System for LTCC Technology
    Vershinin, D., I
    Khusainov, I. N.
    Makarov, N. A.
    [J]. INORGANIC MATERIALS, 2021, 57 (09) : 929 - 936
  • [37] Effect of SiO2/BaO ratio on sintering behavior, crystallization behavior, and properties of SrO-BaO-B2O3-SiO2 glass-ceramics
    Zhang, Bing
    He, Feng
    Cao, Xiuhua
    Ren, Haidong
    Yan, Dongyang
    Xie, Junlin
    [J]. CERAMICS INTERNATIONAL, 2021, 47 (13) : 19043 - 19051
  • [38] Effect of Bi4B2O9 addition on the sintering temperature and microwave dielectric properties of BaO-Nd2O3-4TiO2 ceramics
    Chen, Xingyu
    Zhang, Weijun
    Bai, Shuxin
    [J]. JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2013, 24 (01) : 224 - 229
  • [39] Sintering Behavior, Phase Composition and Microwave Dielectric Characteristics of Mg4Nb2O9 Ceramics Doped with ZnO-B2O3-SiO2 Glass
    Fu, Zhifen
    He, Ying
    [J]. INTEGRATED FERROELECTRICS, 2021, 221 (01) : 161 - 167
  • [40] Sintering behavior and microwave dielectric properties of SiO2–MgO–Al2O3–TiO2 ceramics
    Kh. A. Nekouee
    R. A. Khosroshahi
    R. Taherzadeh Mousavian
    N. Ehsani
    [J]. Journal of Materials Science: Materials in Electronics, 2016, 27 : 3570 - 3575