Low-Cost Carbazole-Based Hole-Transport Material for Highly Efficient Perovskite Solar Cells

被引:44
|
作者
Chen, Zhiliang [1 ]
Li, Hui [2 ]
Zheng, Xiaolu [1 ]
Zhang, Qi [1 ]
Li, Zhanfeng [2 ]
Hao, Yuying [2 ]
Fang, Guojia [1 ]
机构
[1] Wuhan Univ, Key Lab Artificial Micro & Nanostruct, Minist Educ China, Sch Phys & Technol, Wuhan 430072, Hubei, Peoples R China
[2] Taiyuan Univ Technol, Key Lab Adv Transducers & Intelligent Control Sys, Minist Educ & Shanxi Prov, Coll Phys & Optoelect, Taiyuan 030024, Shanxi, Peoples R China
基金
中国国家自然科学基金;
关键词
carbazoles; hole-transport material; nitrogen heterocycles; perovskite; solar cells; COPPER PHTHALOCYANINE; HIGH-PERFORMANCE; LAYERS;
D O I
10.1002/cssc.201700678
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A low-cost carbazole-based small-molecule material, 1,3,6,8-tetra(N,N-p-dimethoxyphenylamino)-9-ethylcarbazole, was designed and synthesized through a facile three-step synthetic route. The material was characterized and applied as a holetransport material (HTM) for low-temperature-processed planar perovskite solar cells (PSCs). Devices based on this new HTM exhibit a high power-conversion efficiency of 17.8% that is comparable to that of PSCs based on the costly 2,2',7,7'-tetrakis[N,N-di(4-methoxyphenyl) amino]-9,9'-spirobifluorene (Spiro-OMeTAD) (18.6%).
引用
收藏
页码:3111 / 3117
页数:7
相关论文
共 50 条
  • [1] Carbazole-based enamine: Low-cost and efficient hole transporting material for perovskite solar cells
    Daskeviciene, Maryte
    Paek, Sanghyun
    Wang, Zhiping
    Malinauskas, Tadas
    Jokubauskaite, Gabriele
    Rakstys, Kasparas
    Cho, Kyung Taek
    Magomedov, Artiom
    Jankauskas, Vygintas
    Ahmad, Shahzada
    Snaith, Henry J.
    Getautis, Vytautas
    Nazeeruddin, Mohammad Khaja
    [J]. NANO ENERGY, 2017, 32 : 551 - 557
  • [2] A low-cost asymmetric carbazole-based hole-transporting material for efficient perovskite solar cells
    Li, Xueqiao
    Sun, Na
    Li, Zhanfeng
    Chen, Jinbo
    Sun, Qinjun
    Wang, Hua
    Hao, Yuying
    [J]. NEW JOURNAL OF CHEMISTRY, 2021, 45 (02) : 735 - 741
  • [3] SFX as a low-cost 'Spiro' hole-transport material for efficient perovskite solar cells
    Maciejczyk, Michal
    Ivaturi, Aruna
    Robertson, Neil
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2016, 4 (13) : 4855 - 4863
  • [4] Carbazole-based hole-transport materials for efficient Perovskite solar cells. A computational study
    Atir, Redouane
    Idrissi, Abdennacer
    Elfakir, Zouhair
    Habsaoui, Amar
    Touhami, Mohamed Ebn
    Bouzakraoui, Said
    [J]. OPTIK, 2022, 257
  • [5] Molecularly engineered hole-transport material for low-cost perovskite solar cells
    Pashaei, Babak
    Bellani, Sebastiano
    Shahroosvand, Hashem
    Bonaccorso, Francesco
    [J]. CHEMICAL SCIENCE, 2020, 11 (09) : 2429 - 2439
  • [6] Low-Cost TiS2 as Hole-Transport Material for Perovskite Solar Cells
    Huckaba, Aron J.
    Gharibzadeh, Saba
    Ralaiarisoa, Maryline
    Roldan-Carmona, Cristina
    Mohammadian, Nasim
    Grancini, Giulia
    Lee, Yonghui
    Amsalem, Patrick
    Plichta, Edward J.
    Koch, Norbert
    Moshaii, Ahmad
    Nazeeruddin, Mohammad Khaja
    [J]. SMALL METHODS, 2017, 1 (10):
  • [7] A carbazole-based dopant-free hole-transport material for perovskite solar cells by increasing the molecular conjugation
    Cai, Bin
    An, Jincheng
    Ge, Mingyao
    Pan, Siqi
    Ji, Wenxi
    Yang, Xichuan
    [J]. ORGANIC ELECTRONICS, 2021, 96
  • [8] Cuprous Oxide as a Potential Low-Cost Hole-Transport Material for Stable Perovskite Solar Cells
    Nejand, Bahram Abdollahi
    Ahmadi, Vahid
    Gharibzadeh, Saba
    Shahverdi, Hamid Reza
    [J]. CHEMSUSCHEM, 2016, 9 (03) : 302 - 313
  • [9] Carbazole-Based Hole-Transport Materials for High-Efficiency and Stable Perovskite Solar Cells
    Gao, Liguo
    Schloemer, Tracy H.
    Zhang, Fei
    Chen, Xihan
    Xiao, Chuanxiao
    Zhu, Kai
    Sellinger, Alan
    [J]. ACS APPLIED ENERGY MATERIALS, 2020, 3 (05) : 4492 - 4498
  • [10] Carbazole-based donor materials with enhanced photovoltaic parameters for organic solar cells and hole-transport materials for efficient perovskite solar cells
    Gul, Shehla
    Hameed, Shanza
    Ans, Muhammad
    Iqbal, Javed
    [J]. JOURNAL OF MOLECULAR MODELING, 2022, 28 (11)