Resonant sum-frequency generation in chiral liquids

被引：11
|
作者：
Belkin, MA
Kulakov, TA
Ernst, KH
Han, SH
Shen, YR [1 ]
机构：
[1] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
[2] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA
来源：
OPTICAL MATERIALS | 2003年 / 21卷 / 1-3期
关键词：
sum-frequency generation; nonlinear optical activity;
D O I：
10.1016/S0925-3467(02)00104-0
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
Sum-frequency generation in chiral liquids is conclusively demonstrated. Enhancement through both electronic and vibrational resonances is observed, providing a novel spectroscopic method for probing molecular chirality. Although the process is electric-dipole allowed, the signal strength is rather weak. This can be understood from the physical mechanism that leads to the chiral nonlinearity. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码：1 / 5
页数：5
相关论文
共 50 条
  • [21] SUM-FREQUENCY GENERATION IN THE XUV
    DINEV, S
    DREISCHUH, A
    OPTICAL AND QUANTUM ELECTRONICS, 1991, 23 (01) : 91 - 97
  • [22] SUM-FREQUENCY GENERATION IN GASES
    COHAN, NV
    HAMEKA, HF
    JOURNAL OF CHEMICAL PHYSICS, 1967, 46 (09): : 3690 - &
  • [23] Toward Chiral sum-frequency spectroscopy
    Ji, Na
    Ostroverkhov, Victor
    Belkin, Mikhail
    Shiu, Ying-Jen
    Shen, Yuen-Ron
    Journal of the American Chemical Society, 2006, 128 (27): : 8845 - 8848
  • [24] Toward chiral sum-frequency spectroscopy
    Ji, Na
    Ostroverkhov, Victor
    Belkin, Mikhail
    Shiu, Ying-Jen
    Shen, Yuen-Ron
    JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2006, 128 (27) : 8845 - 8848
  • [25] High spatial resolution collinear chiral sum-frequency generation microscopy
    Ji, Ziheng
    Yu, Wentao
    Dong, Dashan
    Yang, Hong
    Liu, Kaihui
    Xiao, Yun-Feng
    Gong, Qihuang
    Song, Qinghai
    Shi, Kebin
    ADVANCED PHOTONICS NEXUS, 2024, 3 (02):
  • [26] NONLINEAR-OPTICAL STUDIES OF SURFACE ADSORBATES BY RESONANT SUM-FREQUENCY GENERATION
    MESSMER, MC
    RICHMOND, GL
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 1994, 207 : 204 - PHYS
  • [27] Sum-frequency vibrational spectroscopy on chiral liquids: A novel technique to probe molecular chirality
    Belkin, MA
    Kulakov, TA
    Ernst, KH
    Yan, L
    Shen, YR
    PHYSICAL REVIEW LETTERS, 2000, 85 (21) : 4474 - 4477
  • [28] A theoretical study of sum-frequency generation for chiral solutions near electronic resonance
    Zheng, Ren-hui
    Wei, Wen-mei
    Shi, Qiang
    PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2015, 17 (31) : 20296 - 20300
  • [29] Femtosecond Vibrational Sum-Frequency Generation Spectroscopy of Chiral Molecules in Isotropic Liquid
    Lee, Taegon
    Rhee, Hanju
    Cho, Minhaeng
    JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2018, 9 (23): : 6723 - 6730
  • [30] Optically active sum-frequency generation as an advanced tool for chiral metallopolymer material
    Taupier, Gregory
    Torres-Werle, Maria
    Boeglin, Alex
    Maisse-Francois, Aline
    Achard, Thierry
    Bellemin-Laponnaz, Stephane
    Dorkenoo, Kokou Dodzi
    APPLIED PHYSICS LETTERS, 2017, 110 (02)
12345