Enhancement of α-oxygen formation and N2O decomposition on Fe/ZSM-5 catalysts by extraframework Al

被引：37
|
作者：
Sun, KQ [1 ]
Zhang, HD [1 ]
Xia, H [1 ]
Lian, YX [1 ]
Li, Y [1 ]
Feng, ZC [1 ]
Ying, PL [1 ]
Li, C [1 ]
机构：
[1] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
来源：
CHEMICAL COMMUNICATIONS | 2004年 / 21期
关键词：
D O I：
10.1039/b408854a
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
The concentration of alpha-oxygen which can oxidize methane to methanol and benzene to phenol at RT, increases linearly with the amount of introduced extraframework Al on Fe/ZSM-5 catalysts prepared by solid-state exchange of FeCl3 and AlCl3 with H-ZSM-5.
引用
收藏
页码：2480 / 2481
页数：2
相关论文
共 50 条
  • [41] The effect of adsorbates on N2O formation in pulsing NO over a Pt/ZSM-5 catalyst
    Rottlander, C
    Andorf, R
    Plog, C
    Krutzsch, B
    Baerns, M
    JOURNAL OF CATALYSIS, 1997, 169 (01) : 400 - 403
  • [42] Nano ZSM-5 type ferrisilicates as novel catalysts for ethylbenzene dehydrogenation in the presence of N2O
    Khatamian, M.
    Khandar, A. A.
    Haghighi, M.
    Ghadiri, M.
    APPLIED SURFACE SCIENCE, 2011, 258 (02) : 865 - 872
  • [43] The mechanism of N2O decomposition on Fe-ZSM-5:: an isotope labeling study
    Pirngruber, GD
    Roy, PK
    CATALYSIS LETTERS, 2004, 93 (1-2) : 75 - 80
  • [44] N2O Decomposition over Fe-ZSM-5 Studied by Transient Techniques
    Prechtl, Petra M.
    Kiwi-Minsker, Lioubov
    Bulushev, Dmitri A.
    Bromley, Bryan K.
    Renken, Albert
    CHEMICAL ENGINEERING & TECHNOLOGY, 2009, 32 (09) : 1403 - 1410
  • [45] Water vapor effects in N2O decomposition over Fe-ZSM-5 catalysts with low iron content
    Ecole Polytechnique Fédérale de Lausanne, LGRC-EPFL, CH-1015, Lausanne, Switzerland
    Ind. Eng. Chem. Res., 2007, 12 (4178-4185):
  • [46] The Mechanism of N2O Decomposition on Fe-ZSM-5: An Isotope Labeling Study
    Gerhard D. Pirngruber
    Pijus K. Roy
    Catalysis Letters, 2004, 93 : 75 - 80
  • [47] Experimental and theoretical studies of N2O decomposition over Fe-ZSM-5.
    Bell, AT
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2002, 223 : U649 - U649
  • [48] The effect of pretreatment on the reactivity of Fe-ZSM-5 catalysts for N2O decomposition:: Dehydroxylation vs. steaming
    Roy, Pijus K.
    Prins, Roel
    Pirngruber, Gerhard D.
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2008, 80 (3-4) : 226 - 236
  • [49] Characterization of active surface oxygen in N2O-activated Fe/ZSM-5
    Wen, G
    Zhang, P
    CHINESE JOURNAL OF INORGANIC CHEMISTRY, 2005, 21 (10) : 1535 - 1540
  • [50] Mechanistic origin of the different activity of Rh-ZSM-5 and Fe-ZSM-5 in N2O decomposition
    Kondratenko, Evgenii V.
    Kondratenko, Vita A.
    Santiago, Marta
    Perez-Ramirez, Javier
    JOURNAL OF CATALYSIS, 2008, 256 (02) : 248 - 258
12345