Correlated Electrons in Optically Tunable Quantum Dots: Building an Electron Dimer Molecule

被引:37
|
作者
Singha, Achintya [1 ,2 ]
Pellegrini, Vittorio [1 ,2 ]
Pinczuk, Aron [3 ,4 ,5 ]
Pfeiffer, Loren N. [6 ,8 ]
West, Ken W. [6 ,8 ]
Rontani, Massimo [7 ]
机构
[1] CNR, NEST, Ist Nanosci, I-56127 Pisa, Italy
[2] Scuola Normale Super Pisa, I-56127 Pisa, Italy
[3] Columbia Univ, Dept Appl Phys, New York, NY 10027 USA
[4] Columbia Univ, Dept Appl Math, New York, NY 10027 USA
[5] Columbia Univ, Dept Phys, New York, NY 10027 USA
[6] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA
[7] CNR, Ist Nanosci, S3, I-41125 Modena, Italy
[8] Alcatel Lucent, Bell Labs, Murray Hill, NJ 07974 USA
基金
美国国家科学基金会;
关键词
MAGNETIC-FIELD; SPECTROSCOPY; EXCITATIONS; SCATTERING; MOTION;
D O I
10.1103/PhysRevLett.104.246802
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We observe the low-lying excitations of a molecular dimer formed by two electrons in a GaAs semiconductor quantum dot in which the number of confined electrons is tuned by optical illumination. By employing inelastic light scattering we identify the intershell excitations in the one-electron regime and the distinct spin and charge modes in the interacting few-body configuration. In the case of two electrons, a comparison with configuration-interaction calculations allows us to link the observed excitations with the breathing mode of the molecular dimer and to determine the singlet-triplet energy splitting.
引用
收藏
页数:4
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