Charge and heat transport in soft nanosystems in the presence of time-dependent perturbations

被引:4
|
作者
Nocera, Alberto [1 ]
Perroni, Carmine Antonio [2 ,3 ]
Ramaglia, Vincenzo Marigliano [2 ,3 ]
Cataudella, Vittorio [2 ,3 ]
机构
[1] Northeastern Univ, Dept Phys, Boston, MA 02115 USA
[2] Univ Naples Federico II, Complesso Univ Monte St Angelo, CNR SPIN, I-80126 Naples, Italy
[3] Univ Naples Federico II, Complesso Univ Monte St Angelo, Dept Phys Ettore Pancini, I-80126 Naples, Italy
来源
关键词
electronic charge quantum pumping; electronic transport theory; nanoelectromechanical systems; thermoelectric properties; time-dependent perturbations; QUANTUM LIMIT; SINGLE; THERMOELECTRICITY; FLOW;
D O I
10.3762/bjnano.7.39
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Background: Soft nanosystems are electronic nanodevices, such as suspended carbon nanotubes or molecular junctions, whose transport properties are modulated by soft internal degrees of freedom, for example slow vibrational modes. Effects of the electron-vibration coupling on the charge and heat transport of soft nanoscopic systems are theoretically investigated in the presence of time-dependent perturbations, such as a forcing antenna or pumping terms between the leads and the nanosystem. A well-established approach valid for non-equilibrium adiabatic regimes is generalized to the case where external time-dependent perturbations are present. Then, a number of relevant applications of the method are reviewed for systems composed by a quantum dot (or molecule) described by a single electronic level coupled to a vibrational mode. Results: Before introducing time-dependent perturbations, the range of validity of the adiabatic approach is discussed showing that a very good agreement with the results of an exact quantum calculation is obtained in the limit of low level occupation. Then, we show that the interplay between the low frequency vibrational modes and the electronic degrees of freedom affects the thermoelectric properties within the linear response regime finding out that the phonon thermal conductance provides an important contribution to the figure of merit at room temperature. Our work has been stimulated by recent experimental results on carbon nanotube electromechanical devices working in the semiclassical regime (resonator frequencies in the megahertz range compared to an electronic hopping frequency of the order of tens of gigahertz) with extremely high quality factors. The nonlinear vibrational regime induced by the external antenna in such systems has been discussed within the non-perturbative adiabatic approach reproducing quantitatively the characteristic asymmetric shape of the current-frequency curves. Within the same set-up, we have proved that the antenna is able to pump sufficient charge close to the mechanical resonance making single-parameter adiabatic charge pumping feasible in carbon nanotube resonators. The pumping mechanism that we observe is different from that acting in the two parameter pumping and, instead, it is based on an important dynamic adjustment of the mechanical motion of the nanotube to the external drive in the weakly nonlinear regime. Finally, stochastic forces induced by quantum and thermal fluctuations due to the electron charging of the quantum dot are shown to affect in a significant way a Thouless charge pump realized with an elastically deformable quantum dot. In this case, the pumping mechanism is also shown to be magnified when the frequency of the external drive is resonant with the proper frequency of the deformable quantum dot. In this regime, the pumping current is not strongly reduced by the temperature, giving a measurable effect. Conclusion: Aim of this review has been to discuss common features of different soft nanosystems under external drive. The most interesting effects induced by time-dependent perturbations are obtained when the external forcing is nearly resonant with the slow vibrational modes. Indeed, not only the external forcing can enhance the electronic response, but it also induces nonlinear regimes where the interplay between electronic and vibrational degrees of freedom plays a major role.
引用
收藏
页码:439 / 464
页数:26
相关论文
共 50 条
  • [21] TIME-DEPENDENT WAVEFUNCTIONS FOR 2 INDEPENDENT PERTURBATIONS
    LEIPERT, TK
    GRANT, DM
    JOURNAL OF CHEMICAL PHYSICS, 1975, 63 (07): : 2775 - 2781
  • [22] Irregular time-dependent perturbations of quantum Hamiltonians
    Robert, Didier
    JOURNAL OF SPECTRAL THEORY, 2016, 6 (04) : 955 - 976
  • [23] Kepler problem with time-dependent and resonant perturbations
    Vrbik, Jan
    JOURNAL OF MATHEMATICAL PHYSICS, 2007, 48 (05)
  • [24] Time-dependent gradient perturbations of fractional Laplacian
    Tomasz Jakubowski
    Karol Szczypkowski
    Journal of Evolution Equations, 2010, 10 : 319 - 339
  • [25] Fermi gas response to time-dependent perturbations
    d'Ambrumenil, N
    Muzykantskii, B
    PHYSICAL REVIEW B, 2005, 71 (04)
  • [26] TIME-DEPENDENT TRANSPORT OF DUST
    HASSAN, MHA
    ELTAYEB, IA
    JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1991, 96 (D5) : 9337 - 9339
  • [27] TIME-DEPENDENT TRANSPORT PROCESS
    PINGIWAN.A
    JOURNAL OF THE FRANKLIN INSTITUTE-ENGINEERING AND APPLIED MATHEMATICS, 1969, 287 (05): : 409 - &
  • [28] Geometric heat pump:Controlling thermal transport with time-dependent modulations
    Zi Wang
    Luqin Wang
    Jiangzhi Chen
    Chen Wang
    Jie Ren
    Frontiers of Physics, 2022, 17 (01) : 150 - 163
  • [29] Geometric heat pump: Controlling thermal transport with time-dependent modulations
    Zi Wang
    Luqin Wang
    Jiangzhi Chen
    Chen Wang
    Jie Ren
    Frontiers of Physics, 2022, 17
  • [30] Geometric heat pump: Controlling thermal transport with time-dependent modulations
    Wang, Zi
    Wang, Luqin
    Chen, Jiangzhi
    Wang, Chen
    Ren, Jie
    FRONTIERS OF PHYSICS, 2022, 17 (01)