The femtosecond fifth-order nonlinear response of nuclear motion in liquids

被引：0
|
作者：
Steffen, T
Duppen, K
机构：
来源：
FEMTOCHEMISTRY: ULTRAFAST CHEMICAL AND PHYSICAL PROCESSES IN MOLECULAR SYSTEMS | 1996年
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D O I：
暂无
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The femtosecond fifth-order nonlinear response of CS2 is measured using nonresonant six-wave mixing. This method provides new information on the dephasing mechanisms of coherently excited nuclear motion that is not accessible in third-order experiments. Our experimental results indicate that the ultrafast librational motion in CS2 is overdamped and predominantly homogeneously broadened. The results deviate from those of Tominaga and Yoshihara and can be explained only partly within the model of Tanimura and Mukamel.
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页码：583 / 586
页数：4
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