High-throughput screening of heterogeneous catalyst under pressurized conditions - Optimization of Cu-Mn oxide catalyst for methanol synthesis

被引:0
|
作者
Omata, K [1 ]
Ishiguro, G [1 ]
Yamada, M [1 ]
机构
[1] Tohoku Univ, Grad Sch Engn, Dept Appl Chem, Aoba Ku, Sendai, Miyagi 9808579, Japan
来源
SEKIYU GAKKAISHI-JOURNAL OF THE JAPAN PETROLEUM INSTITUTE | 2000年 / 43卷 / 04期
关键词
reactor; activity; mixed oxide catalyst; methanol; combinatorial chemistry; high-throughput screening;
D O I
暂无
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
High-throughput screening was performed to optimize the Cu/Mn ratio of Cu-Mn oxide catalyst for methanol synthesis from syngas at 1 MPa and 523 K. The autoclave equipped with twelve catalyst beds was connected to a conventional high-pressure gas flow apparatus. Identical temperature and identical space velocity over the 12 catalyst beds was ensured. The catalyst showed the same activity as that of the catalyst used in the conventional test, indicating the possibility of high efficiency catalyst screening under conventional testing conditions.
引用
收藏
页码:317 / 319
页数:3
相关论文
共 50 条
  • [31] Effects of the Calcination and Reduction Conditions on a Cu/ZnO Methanol Synthesis Catalyst
    Shin-ichiro Fujita
    Shuhei Moribe
    Yoshinori Kanamori
    Nobutsune Takezawa
    Reaction Kinetics and Catalysis Letters, 2000, 70 : 11 - 16
  • [32] A novel Cu-Mn/Ca-Zr catalyst for the synthesis of methyl formate from syngas
    Zhao, Haijun
    Lin, Minggui
    Fang, Kegong
    Zhou, Juan
    Liu, Ziyu
    Zeng, Gaofeng
    Sun, Yuhan
    RSC ADVANCES, 2015, 5 (83): : 67630 - 67637
  • [33] A thermostable cu-mn based catalyst for high temperature water-gas-shift reaction
    Liu, QS
    He, RX
    Cu, XL
    Zhi, KD
    Ma, WP
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2005, 230 : U1675 - U1675
  • [34] Comparison of the methods for preparing a cordierite monolith-supported Cu-Mn mixed-oxide catalyst
    Wu, Dongfang
    Li, Wangbing
    Gao, Rui
    JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY, 2014, 89 (10) : 1559 - 1564
  • [35] QM-Mechanism-Based Hierarchical High-Throughput in Silico Screening Catalyst Design for Ammonia Synthesis
    An, Qi
    Shen, Yidi
    Fortunelli, Alessandro
    Goddard, William A., III
    JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2018, 140 (50) : 17702 - 17710
  • [36] Application of polymerization kinetic Modeling in high-throughput screening of catalyst systems for productivity
    Beigzadeh, Daryoosh
    MACROMOLECULAR REACTION ENGINEERING, 2007, 1 (03) : 331 - 337
  • [37] A high-throughput catalyst synthesis system for Ag-based catalysts
    Deng, Zhuoran
    Zhao, Liqiang
    Cheng, Daojian
    REVIEW OF SCIENTIFIC INSTRUMENTS, 2022, 93 (11):
  • [38] Ball-milling synthesized hydrotalcite supported Cu-Mn mixed oxide under solvent-free conditions: an active catalyst for aerobic oxidative synthesis of 2-acylbenzothiazoles and quinoxalines
    Meng, Xu
    Bi, Xiuru
    Yu, Chaoying
    Chen, Gexin
    Chen, Baohua
    Jing, Zhenqiang
    Zhao, Peiqing
    GREEN CHEMISTRY, 2018, 20 (20) : 4638 - 4644
  • [39] High-throughput testing of heterogeneous catalyst libraries using array microreactors and mass spectrometry
    Senkan, S
    Krantz, K
    Ozturk, S
    Zengin, V
    Onal, I
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 1999, 38 (18) : 2794 - 2799
  • [40] Preparation and evaluation of Cu-Mn/Ca-Zr catalyst for methyl formate synthesis from syngas
    Zhao, Haijun
    Lin, Minggui
    Fang, Kegong
    Zhou, Juan
    Sun, Yuhan
    APPLIED CATALYSIS A-GENERAL, 2016, 514 : 276 - 283