Optical Second Harmonic Generation of Single Metallic Nanoparticles Embedded in a Homogeneous Medium

被引：222
|
作者：
Butet, Jeremy [1 ]
Duboisset, Julien [1 ]
Bachelier, Guillaume [1 ]
Russier-Antoine, Isabelle [1 ]
Benichou, Emmanuel [1 ]
Jonin, Christian [1 ]
Brevet, Pierre-Francois [1 ]
机构：
[1] Univ Lyon 1, Spectrometrie Ion & Mol Lab, CNRS, UMR 5579, F-69622 Villeurbanne, France
来源：
NANO LETTERS | 2010年 / 10卷 / 05期
关键词：
Single nanoparticle; gold; plasmonics; nonlinear optics; second harmonic generation; finite element method simulation; HYPER-RAYLEIGH-SCATTERING; GOLD NANOPARTICLES; COPPER NANOPARTICLES; MOLECULE DETECTION; NANODIMERS; RESPONSES; LIMIT;
D O I：
10.1021/nl1000949
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
We report the optical second harmonic generation from individual 150 nm diameter gold nanoparticles dispersed in gelatin. The quadratic hyperpolarizability of the particles is determined and the input polarization dependence of the second harmonic intensity obtained. These results are found in excellent agreement with ensemble measurements and finite element simulations. These results open up new perspectives for the investigation of the nonlinear optical properties of noble metal nanoparticles.
引用
收藏
页码：1717 / 1721
页数：5
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