Interplay between multiple charge-density waves and the relationship with superconductivity in PdxHoTe3

HoTe3, a member of the rare-earth tritelluride (RTe3) family, and its Pd-intercalated compounds, PdxHoTe3, where superconductivity (SC) sets in as the charge-density wave (CDW) transition is suppressed by the intercalation of a small amount of Pd, are investigated using angle-resolved photoemission spectroscopy (ARPES) and electrical resistivity. Two incommensurate CDWs with perpendicular nesting vectors are observed in HoTe3 at low temperatures. With a slight Pd intercalation (x = 0.01), the large CDW gap decreases and the small one increases. The momentum dependence of the gaps along the inner Fermi surface (FS) evolves from orthorhombicity to near tetragonality, manifesting the competition between two CDW orders. At x = 0.02, both CDW gaps decrease with the emergence of SC. Further increasing the content of Pd for x = 0.04 will completely suppress the CDW instabilities and give rise to the maximal SC order. The evolution of the electronic structures and electron-phonon couplings (EPCs) of the multiple CDWs upon Pd intercalation are carefully scrutinized. We discuss the interplay between multiple CDW orders, and the competition between CDW and SC in detail.