Mean-Field Caging in a Random Lorentz Gas

被引:11
|
作者
Biroli, Giulio [1 ]
Charbonneau, Patrick [2 ,3 ]
Hu, Yi [2 ]
Ikeda, Harukuni [4 ]
Szamel, Grzegorz [5 ]
Zamponi, Francesco [1 ]
机构
[1] Univ Paris, Lab Phys Ecole Normale Super, ENS, Univ PSL,CNRS,Sorbonne Univ, F-75005 Paris, France
[2] Duke Univ, Dept Chem, Durham, NC 27708 USA
[3] Duke Univ, Dept Phys, Durham, NC 27708 USA
[4] Univ Tokyo, Grad Sch Arts & Sci, Tokyo 1538902, Japan
[5] Colorado State Univ, Dept Chem, Ft Collins, CO 80523 USA
来源
JOURNAL OF PHYSICAL CHEMISTRY B | 2021年 / 125卷 / 23期
基金
美国国家科学基金会;
关键词
VOID PERCOLATION PROBLEM; GLASS-TRANSITION; DYNAMICAL THEORY; LOCALIZATION; STORAGE; MODEL;
D O I
10.1021/acs.jpcb.1c02067
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The random Lorentz gas (RLG) is a minimal model of both percolation and glassiness, which leads to a paradox in the infinite-dimensional, d. 8 limit: the localization transition is then expected to be continuous for the former and discontinuous for the latter. As a putative resolution, we have recently suggested that, as d increases, the behavior of the RLG converges to the glassy description and that percolation physics is recovered thanks to finited perturbative and nonperturbative (instantonic) corrections [Biroli et al. Phys. Rev. E 2021, 103, L030104]. Here, we expand on the d -> infinity physics by considering a simpler static solution as well as the dynamical solution of the RLG. Comparing the 1/d correction of this solution with numerical results reveals that even perturbative corrections fall out of reach of existing theoretical descriptions. Comparing the dynamical solution with the mode-coupling theory (MCT) results further reveals that, although key quantitative features of MCT are far off the mark, it does properly capture the discontinuous nature of the d ->infinity RLG. These insights help chart a path toward a complete description of finite-dimensional glasses.
引用
收藏
页码:6244 / 6254
页数:11
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