Effect of ambient condition for coaxial dielectric barrier discharge reactor on CO2 reforming of CH4 to syngas

被引：22
|
作者：
Duc Ba Nguyen [1 ]
Lee, Won Gyu [1 ]
机构：
[1] Kangwon Natl Univ, Dept Chem Engn, Chunchon 200701, Kangwon, South Korea
来源：
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY | 2014年 / 20卷 / 03期
基金：
新加坡国家研究基金会;
关键词：
Syngas; Dielectric barrier discharge; Air ambient; Electrical insulating oil; Plasma reaction; FREQUENCY PULSED PLASMA; CARBON-DIOXIDE; SYNTHESIS GAS; LOW-TEMPERATURE; METHANE; CONVERSION; CATALYSTS; HYDROCARBONS;
D O I：
10.1016/j.jiec.2013.06.031
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
A coaxial dielectric barrier discharge reactor was used for the CO2 reforming of CH4 to syngas. The reactor was operated under two ambient conditions for comparison, namely, immersion in electrical insulating oil and total exposure in an air ambient. Immersion of the reactor in insulating oil increased the electrical power efficiency into the generation of plasma discharge due to the prevention of micro-arcing on the reactor surface. Operation in the insulating oil bath showed higher conversion and selectivity of major reactants and products rate than operation in an air ambient. (C) 2013 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码：972 / 978
页数：7
相关论文
共 50 条
  • [21] Effect of support on performance of Ni based catalysts for CH4/CO2 reforming to syngas
    Li, Xian-Cai
    Li, Shui-Gen
    Yang, Yi-Feng
    Cao, Xiao-Hua
    Xiandai Huagong/Modern Chemical Industry, 2007, 27 (08): : 30 - 33
  • [22] Integrated CO2 Capture and Dry Reforming of CH4 to Syngas: A Review
    Bhaskaran, Aathira
    Singh, Satyapaul A.
    Reddy, Benjaram M.
    Roy, Sounak
    LANGMUIR, 2024, 40 (29) : 14766 - 14778
  • [23] Simultaneous Generation of Syngas and Multiwalled Carbon Nanotube via CH4/CO2 Reforming with Spark Discharge
    Chung, Wei-Chieh
    Chang, Moo-Been
    ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2017, 5 (01): : 206 - 212
  • [24] Heating effect of plasma catalytic reaction on the CH4 reforming of CO2 over Ni/γ-Al2O3 catalyst in dielectric-barrier discharge reactor
    Lee, Hwaung
    Song, Hyung Keun
    Min, Byoung Ryul
    CHEMISTRY LETTERS, 2006, 35 (06) : 646 - 647
  • [25] SPECTROSCOPIC CHARACTERIZATION OF A CH4 PLUS CO2 PLASMA OBTAINED BY DIELECTRIC BARRIER DISCHARGE
    MOTRET, O
    MASSEREAU, V
    NIKRAVECH, M
    HILBERT, C
    POUVESLE, JM
    CHAPELLE, J
    ANNALES DE PHYSIQUE, 1994, 19 (05) : 157 - 158
  • [26] CO2 Hydrogenation by CH4 in a Dielectric Barrier Discharge: Catalytic Effects of Nickel and Copper
    Scapinello, Marco
    Martini, Luca Matteo
    Tosi, Paolo
    PLASMA PROCESSES AND POLYMERS, 2014, 11 (07) : 624 - 628
  • [27] CO2 reforming of CH4 to syngas over nickel-based catalysts
    Qin, Zuzeng
    Chen, Jie
    Xie, Xinling
    Luo, Xuan
    Su, Tongming
    Ji, Hongbing
    ENVIRONMENTAL CHEMISTRY LETTERS, 2020, 18 (04) : 997 - 1017
  • [28] Dry Reforming of CH4 With CO2 to Generate Syngas by Combined Plasma Catalysis
    Pan, Kuan Lun
    Chung, Wei Chieh
    Chang, Moo Been
    IEEE TRANSACTIONS ON PLASMA SCIENCE, 2014, 42 (12) : 3809 - 3818
  • [29] CO2 reforming of CH4 to syngas over nickel-based catalysts
    Zuzeng Qin
    Jie Chen
    Xinling Xie
    Xuan Luo
    Tongming Su
    Hongbing Ji
    Environmental Chemistry Letters, 2020, 18 : 997 - 1017
  • [30] Role of support in CO2 reforming of CH4 to syngas over Ni catalysts
    Ruckenstein, E
    Hu, YH
    JOURNAL OF CATALYSIS, 1996, 162 (02) : 230 - 238
12345