Significant promotion effect of carbon nanotubes on the electrocatalytic activity of supported Pd NPs for ethanol oxidation reaction of fuel cells: the role of inner tubes

被引:30
|
作者
Zhang, Jin [1 ,2 ]
Cheng, Yi [1 ,2 ]
Lu, Shanfu [3 ]
Jia, Lichao [1 ,2 ]
Shen, Pei Kang [4 ]
Jiang, San Ping [1 ,2 ]
机构
[1] Curtin Univ, Fuels & Energy Technol Inst, Perth, WA 6102, Australia
[2] Curtin Univ, Dept Chem Engn, Perth, WA 6102, Australia
[3] Beihang Univ, Sch Chem & Environm, Beijing 100191, Peoples R China
[4] Sun Yat Sen Univ, Sch Phys & Engn, Adv Energy Mat Res Lab, Guangzhou 510275, Guangdong, Peoples R China
关键词
FORMIC-ACID OXIDATION; OXYGEN REDUCTION; PALLADIUM NANOPARTICLES; RAMAN-SPECTROSCOPY; CATALYSTS; METHANOL; ELECTROOXIDATION; ALCOHOL; MECHANISM; PLATINUM;
D O I
10.1039/c4cc06185c
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The inner tubes of carbon nanotubes (CNTs) have a significant promotion effect on the electrocatalytic activity of Pd nanoparticles (NPs) for the ethanol oxidation of direct alcohol fuel cells (DAFCs) and Pd NPs supported on CNTs with 3-7 walls show a much higher activity as compared to that supported on typical single-walled and multi-walled CNTs.
引用
收藏
页码:13732 / 13734
页数:3
相关论文
共 34 条
  • [1] Carbon nanotubes supported oxygen reduction reaction catalysts: role of inner tubes
    Tian Tian
    Yi Cheng
    Zhenfan Sun
    Kai Huang
    Ming Lei
    Haolin Tang
    [J]. Advanced Composites and Hybrid Materials, 2023, 6
  • [2] Carbon nanotubes supported oxygen reduction reaction catalysts: role of inner tubes
    Tian, Tian
    Cheng, Yi
    Sun, Zhenfan
    Huang, Kai
    Lei, Ming
    Tang, Haolin
    [J]. ADVANCED COMPOSITES AND HYBRID MATERIALS, 2023, 6 (01)
  • [3] Hollow Graphitized Carbon Nanocage Supported Pd Catalyst with Excellent Electrocatalytic Activity for Ethanol Oxidation
    Zhang, Qiang
    Jiang, Liang
    Wang, Hua
    Liu, Jinglei
    Zhang, Junfeng
    Zheng, Yiqun
    Li, Fengting
    Yao, Chenxue
    Hou, Shifeng
    [J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2018, 6 (06): : 7507 - 7514
  • [4] The Beneficial Role of the Cometals Pd and Au in the Carbon-Supported PtPdAu Catalyst Toward Promoting Ethanol Oxidation Kinetics in Alkaline Fuel Cells: Temperature Effect and Reaction Mechanism
    Datta, Jayati
    Dutta, Abhijit
    Mukherjee, Sanjeev
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2011, 115 (31): : 15324 - 15334
  • [5] Electrocatalytic activity of multi-walled carbon nanotubes-supported PtxPdy catalysts prepared by a pyrolysis process toward ethanol oxidation reaction
    Ding, Keqiang
    Wang, Yahui
    Yang, Hongwei
    Zheng, Chunbao
    YanliCao
    Wei, Huige
    Wang, Yiran
    Guo, Zhanhu
    [J]. ELECTROCHIMICA ACTA, 2013, 100 : 147 - 156
  • [6] Effect of nitrogen-containing functionalization on the electrocatalytic activity of PtRu nanoparticles supported on carbon nanotubes for direct methanol fuel cells
    Cheng, Yi
    Xu, Changwei
    Shen, Pei Kang
    Jiang, San Ping
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2014, 158 : 140 - 149
  • [7] Carbon-Nanotubes-Supported Pd Nanoparticles for Alcohol Oxidations in Fuel Cells: Effect of Number of Nanotube Walls on Activity
    Zhang, Jin
    Lu, Shanfu
    Xiang, Yan
    Shen, Pei Kang
    Liu, Jian
    Jiang, San Ping
    [J]. CHEMSUSCHEM, 2015, 8 (17) : 2956 - 2966
  • [8] Enhanced electrocatalytic activity of carbon-supported MnOx/Ru catalysts for methanol oxidation in fuel cells
    Rebello, JS
    Samant, PV
    Figueiredo, JL
    Fernandes, JB
    [J]. JOURNAL OF POWER SOURCES, 2006, 153 (01) : 36 - 40
  • [9] A beehive-shaped Pd and Ni Nanoparticle Composite Showing Significant Electrocatalytic Activity Towards Ethanol Oxidation Reaction (EOR)
    Ding, Keqiang
    Shi, Fujuan
    Zhang, Dongyue
    Li, Boxia
    Chen, Jiasheng
    Di, Mengyao
    Van, Mengying
    Wang, Hui
    [J]. INTERNATIONAL JOURNAL OF ELECTROCHEMICAL SCIENCE, 2022, 17 (04):
  • [10] PtRu catalysts supported on heteropolyacid and chitosan functionalized carbon nanotubes for methanol oxidation reaction of fuel cells
    Cui, Zhiming
    Li, Chang Ming
    Jiang, San Ping
    [J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2011, 13 (36) : 16349 - 16357