Quantification of NO2 and SO2 emissions from the Houston Ship Channel and Texas City industrial areas during the 2006 Texas Air Quality Study

被引:28
|
作者
Rivera, Claudia [1 ]
Mellqvist, Johan [1 ]
Samuelsson, Jerker [1 ]
Lefer, Barry [2 ]
Alvarez, Sergio [3 ]
Patel, Monica R. [2 ]
机构
[1] Chalmers Univ Technol, SE-41296 Gothenburg, Sweden
[2] Univ Houston, Dept Geosci, Houston, TX 77004 USA
[3] Baylor Univ, Inst Air Sci, Waco, TX 76798 USA
关键词
ABSORPTION CROSS-SECTIONS; VOLATILE ORGANIC-COMPOUNDS; TEMPERATURE-DEPENDENCE; TROPOSPHERIC NITROGEN; HYDROCARBON EMISSIONS; AIRBORNE MEASUREMENTS; OZONE FORMATION; FORMALDEHYDE; URBAN; PLUMES;
D O I
10.1029/2009JD012675
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
In August-September 2006, as part of the Second Texas Air Quality Study, NO2 and SO2 emissions from the Houston Ship Channel and Texas City industrial areas were quantified using mobile mini-differential optical absorption spectroscopy instruments. The measured NO2 emissions from the Houston Ship Channel and Texas City industrial areas were 2542 and 452 kg h(-1), respectively, yielding NOx emissions 70% and 43%, respectively, above the reported inventory values. Quantified SO2 emissions from the Houston Ship Channel area were 1749 kg h(-1) and were found to be 34% above the values reported in the inventory. Short-term variability of NO2 and SO2 emissions was found at the Houston Ship Channel. On 31 August 2006, a plume was detected at the HSC during three consecutive measurements, yielding a HCHO flux of 481 kg h(-1). This event has been mainly attributed to photochemical production.
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页数:10
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