We investigate the magnetic coupling across the antiferromagnetic-antiferromagnetic (AFM-AFM) interface for the prototypical CoO-NiO bilayer system where the bulk Neel temperature (T- N ) of NiO is higher than that of CoO. Using the temperature-dependent exchange-scattered electron intensities from the surface AFM lattice, the surface T- N of CoO was estimated as a function of the CoO/NiO film thicknesses. Our results show that the surface T- N of CoO layers is enhanced significantly from its bulk T- N value and approaching the T- N of the NiO layers, as the thickness of the CoO layers is reduced to the monolayer limit. Thus, thinner CoO layers are found to have higher T- N than thicker layers on NiO, contrasting with the expected finite-size behavior. In addition to the short-range magnetic exchange coupling at the CoO-NiO interface, we observe the existence of a longer-range magnetic coupling across the interface, mediated by the magnetic correlations. Thus, the magnetic proximity effect is attributed to a combination of a short-range and a weaker long-range magnetic coupling, explaining the long AFM order propagation length in AFM-AFM superlattices and bilayers. Further, our results indicate a new approach to tune the AFM Neel temperature by varying the individual layer thickness of the bilayer system through the magnetic proximity effect.
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Univ Tokyo, Dept Adv Mat Sci, Kashiwa, Chiba 2778561, JapanUniv Tokyo, Dept Adv Mat Sci, Kashiwa, Chiba 2778561, Japan
Watanabe, Yoshito
Gen, Masaki
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Univ Tokyo, Dept Adv Mat Sci, Kashiwa, Chiba 2778561, Japan
RIKEN, Ctr Emergent Matter Sci CEMS, Wako, Saitama 3510198, JapanUniv Tokyo, Dept Adv Mat Sci, Kashiwa, Chiba 2778561, Japan
Gen, Masaki
Kurumaji, Takashi
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Univ Tokyo, Dept Adv Mat Sci, Kashiwa, Chiba 2778561, JapanUniv Tokyo, Dept Adv Mat Sci, Kashiwa, Chiba 2778561, Japan