The Rechargeable Aluminum Battery: Opportunities and Challenges

被引:332
|
作者
Yang, Huicong [1 ,2 ]
Li, Hucheng [1 ,2 ]
Li, Juan [3 ]
Sun, Zhenhua [1 ,2 ]
He, Kuang [1 ,2 ]
Cheng, Hui-Ming [1 ,2 ,4 ]
Li, Feng [1 ,2 ]
机构
[1] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Liaoning, Peoples R China
[2] Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Liaoning, Peoples R China
[3] Jilin Univ, Coll Phys, Changchun 130012, Jilin, Peoples R China
[4] Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen 518055, Peoples R China
基金
中国国家自然科学基金;
关键词
Coulombic interaction; electrolytes; interface reactions; rechargeable aluminum batteries; LITHIUM METAL ANODE; HIGH-PERFORMANCE; ION BATTERY; CATHODE MATERIAL; ELECTROCHEMICAL INTERCALATION; LIQUID ELECTROLYTES; ANION INTERCALATION; SULFUR BATTERY; DOPED CARBON; HIGH-VOLTAGE;
D O I
10.1002/anie.201814031
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Aluminum battery systems are considered as a system that could supplement current lithium batteries due to the low cost and high volumetric capacity of aluminum metal, and the high safety of the whole battery system. However, first the use of ionic liquid electrolytes leading to AlCl4- instead of Al3+, the different intercalation reagents, the sluggish solid diffusion process and the fast capacity fading during cycling in aluminum batteries all need to be thoroughly explored. To provide a good understanding of the opportunities and challenges of the newly emerging aluminum batteries, this Review discusses the reaction mechanisms and the difficulties caused by the trivalent reaction medium in electrolytes, electrodes, and electrode-electrolyte interfaces. It is hoped that the Review will stimulate scientists and engineers to develop more reliable aluminum batteries.
引用
收藏
页码:11978 / 11996
页数:19
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