Neutron polarization analysis on the multiferroic TbMn2O5

被引:4
|
作者
Chang, L. J. [1 ]
Su, Y. [2 ]
Schweika, W. [3 ]
Brueckel, Th. [2 ,3 ]
Chen, Y. Y. [4 ]
Jang, D. S. [5 ,6 ]
Liu, R. S. [5 ,6 ]
机构
[1] Natl Tsing Hua Univ, Nucl Sci & Technol Dev Ctr, Hsinchu 30013, Taiwan
[2] Forschungszentrum Julich, Inst Festkorperforsch, Outstn FRM II,JCNS, D-85747 Garching, Germany
[3] Forschungszentrum Julich, Inst Festkorperforsch, D-52425 Julich, Germany
[4] Acad Sinica, Inst Phys, Taipei 115, Taiwan
[5] Natl Taiwan Univ, Dept Chem, Taipei 106, Taiwan
[6] Natl Taiwan Univ, Ctr Nano Storage Res, Taipei 106, Taiwan
关键词
Multiferroics; Neutron diffraction; Specific heat; FERROELECTRIC POLARIZATION; SCATTERING; REVERSAL;
D O I
10.1016/j.physb.2009.06.011
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Polycrystalline TbMn2O5 was prepared by the standard solid-state reaction method and characterized by powder X-ray diffraction and magnetization to assure it is of single phase. Heat capacity measurements on the compound reveal an antiferromagnetic phase transition at similar to 45 K. A broad peak below similar to 6 K in the heat capacity measurements corresponds to the crossover transition of Tb3+ ordering. To confirm these magnetic orderings, neutron powder diffractions on TbMn2O5 with XYZ neutron polarization analysis were performed at the diffuse neutron scattering (DNS) spectrometer, FRJ-II, by using neutron wavelength of 4.8 angstrom in the temperature range of 1.8-250 K. Magnetic scattering was separated from nuclear coherent and spin incoherent scattering contributions. Long-range ordered magnetic peaks were observed below similar to 39 K which is consistent with the heat capacity results. The drastic increasing intensities below similar to 6 K indicate the ferromagnetic transition in Tb3+ orderings. (C) 2009 Elsevier B.V. All rights reserved.
引用
收藏
页码:2517 / 2519
页数:3
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