Enhanced wood-derived photothermal evaporation system by in-situ incorporated lignin carbon quantum dots

被引:95
|
作者
Chao, Weixiang [1 ]
Li, Yudong [1 ]
Sun, Xiaohan [1 ]
Cao, Guoliang [2 ]
Wang, Chengyu [1 ]
Ho, Shih-Hsin [2 ]
机构
[1] Northeast Forestry Univ, Mat Sci & Engn Coll, Key Lab Biobased Mat Sci & Technol, Minist Educ, Harbin 150040, Peoples R China
[2] Harbin Inst Technol, Sch Environm, State Key Lab Urban Water Resources & Environm, Harbin 150040, Peoples R China
基金
中国国家自然科学基金;
关键词
Photothermal evaporation; Seawater desalination; Simulation and numerical modelling; Carbon quantum dots; Wood-based resources utilization; HIGHLY EFFICIENT; STEAM-GENERATION; HIGH-PERFORMANCE; ONE SUN; SOLAR; MEMBRANE; DESALINATION; CONVERSION; STRATEGY; BIOMASS;
D O I
10.1016/j.cej.2020.126703
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Photothermal evaporation and desalination via renewable solar energy has promising potential to alleviate freshwater scarcity. However, recent reported systems usually lack sufficient environmental compatibility, ecological security, and energy-saving concern. Here, a novel and green photothermal evaporation system with ecological and economic advantages was designed. An evaporation performance of 1.18 kg.m(-2) (1.09 kg.m(-2).h(-1)) with up to 79.5% efficiency at one sun illumination (1 kW.m(-2)) was achieved. More importantly, a series of simulation and numerical modelling was synchronously developed to analyze in-depth the main factors that affect water transportation and evaporation processes. The channel size, temperature distribution, and formed gradient were carefully investigated and discussed. Notably, this system exhibited satisfactory repeatability and stability. In addition, only a few photothermal components are required in this system, which will also bring a significant economic merit. Taken together, this work successfully provides new insights into developing a sustainable photothermal evaporation system with ecologically friendly property and satisfactory performance in practical application. Moreover, it also reveals the corresponding water transportation and photothermal evaporation mechanisms, and maximizes the evaporation efficiency.
引用
收藏
页数:12
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