Role of bending in the dissociation of selective resonant inner-shell excitation as observed in CO2 -: art. no. 050701

被引:65
|
作者
Morin, P
Simon, M
Miron, C
Leclercq, N
Kukk, E
Bozek, JD
Berrah, N
机构
[1] Univ Paris 11, LURE, F-91405 Orsay, France
[2] CENS, CEA, DRECAM, SPAM, F-91191 Gif Sur Yvette, France
[3] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA
[4] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA
来源
PHYSICAL REVIEW A | 2000年 / 61卷 / 05期
关键词
D O I
10.1103/PhysRevA.61.050701
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Combining high-resolution electron spectroscopy with electron-ion coincidence data, we have been able to show the role of bending excitation in the dissociation of CO2 after C 1s-->Pi(u) resonant excitation. We demonstrate that the predissociation of the dominating A state created through participator decay is not constant along the resonance profile. The interpretation is based on a preferential excitation of high levels of the bending mode at low-photon-energy side of the resonance, which favors the O+ + CO decay channel.
引用
收藏
页数:4
相关论文
共 50 条
  • [31] On error estimation in atmospheric CO2 inversions -: art. no. 4635
    Engelen, RJ
    Denning, AS
    Gurney, KR
    JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D22)
  • [32] Distribution of anthropogenic CO2 in the Pacific Ocean -: art. no. 1083
    Sabine, CL
    Feely, RA
    Key, RM
    Bullister, JL
    Millero, FJ
    Lee, K
    Peng, TH
    Tilbrook, B
    Ono, T
    Wong, CS
    GLOBAL BIOGEOCHEMICAL CYCLES, 2002, 16 (04)
  • [33] Interannual variability in the global uptake of CO2 -: art. no. 1059
    Bates, NR
    GEOPHYSICAL RESEARCH LETTERS, 2002, 29 (05) : 3 - 1
  • [34] Dissociative recombination of the cation and dication of CO2 -: art. no. 022708
    Seiersen, K
    Al-Khalili, A
    Heber, O
    Jensen, MJ
    Nielsen, IB
    Pedersen, HB
    Safvan, CP
    Andersen, LH
    PHYSICAL REVIEW A, 2003, 68 (02):
  • [35] Linear polarization of the 2p53s→2p6 lines following the inner-shell photoionization of sodiumlike ions -: art. no. 042720
    Inal, MK
    Surzhykov, A
    Fritzsche, S
    PHYSICAL REVIEW A, 2005, 72 (04):
  • [36] CO2 molecule as a quantum realization of the 1:1:2 resonant swing-spring with monodromy -: art. no. 024302
    Cushman, RH
    Dullin, HR
    Giacobbe, A
    Holm, DD
    Joyeux, M
    Lynch, P
    Sadovskií, DA
    Zhilinskií, BI
    PHYSICAL REVIEW LETTERS, 2004, 93 (02) : 024302 - 1
  • [37] Interference effects between 2p photoionization and resonant Auger decay channels at 2s-1np (n=4,5) inner-shell resonances in Ar -: art. no. 042702
    Sankari, R
    Kivimäki, A
    Huttula, M
    Matila, T
    Aksela, H
    Aksela, S
    Coreno, M
    Turri, G
    Camilloni, R
    de Simone, M
    Prince, KC
    PHYSICAL REVIEW A, 2002, 65 (04): : 427021 - 427026
  • [38] Atmospheric CO2 balance:: The role of Arctic sea ice -: art. no. L05121
    Semiletov, I
    Makshtas, A
    Akasofu, SI
    Andreas, EL
    GEOPHYSICAL RESEARCH LETTERS, 2004, 31 (05)
  • [39] Virtual-state effects on elastic scattering and vibrational excitation of CO2 by electron impact -: art. no. 040701
    Mazevet, S
    Morrison, MA
    Morgan, LA
    Nesbet, RK
    PHYSICAL REVIEW A, 2001, 64 (04): : 4
  • [40] Negative ion formation following inner-shell photoexcitation in CO2 studied by velocity imaging spectroscopy
    Hikosaka, Y.
    Kaneyasu, T.
    Tamenori, Y.
    Shigemasa, E.
    JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2007, 156 : 284 - 288