Estimation of ecotoxicity of petroleum hydrocarbon mixtures in soil based on HPLC-GCXGC analysis

被引：29
|
作者：
Mao, Debin [1 ,2 ]
Lookman, Richard [1 ]
Van De Weghe, Hendrik [1 ]
Weltens, Reinhilde [1 ]
Vanermen, Guido [1 ]
De Brucker, Nicole [1 ]
Diels, Ludo [1 ,2 ]
机构：
[1] Flemish Inst Technol Res VITO, B-2400 Mol, Belgium
[2] Univ Antwerp, Dept Biol, B-2610 Antwerp, Belgium
来源：
CHEMOSPHERE | 2009年 / 77卷 / 11期
关键词：
Toxicity; TPH; Aromatic petroleum hydrocarbons; Leaching water; Comprehensive two-dimensional gas chromatography; 2-DIMENSIONAL GAS-CHROMATOGRAPHY; OIL CONTAMINATED SOILS; RISK-ASSESSMENT; CRUDE OILS; BIOREMEDIATION; BIODEGRADATION; ENVIRONMENT; EARTHWORMS; TOXICITY; NAPLS;
D O I：
10.1016/j.chemosphere.2009.10.004
中图分类号：
X [环境科学、安全科学];
学科分类号：
08 ; 0830 ;
摘要：
Detailed HPLC-GCXGC/FID (high performance liquid chromatography followed by comprehensive two-dimensional gas chromatography with flame-ionization detection) analysis of oil-contaminated soils was performed to interpret results of selected acute ecotoxicity assays. For the five ecotoxicity assays tested, plant seed germination and Microtox (R) were selected as most sensitive for evaluating ecotoxicity of the oil in the soil phase and in the leaching water, respectively. The measured toxicity for cress when testing the soil samples did not correspond to TPH concentration in the soil. A detailed chemical composition analysis of the oil contamination using HPLC-GCXGC/FID allows to better predict the ecotoxicological risk and leaching potential of petroleum hydrocarbons in soil. Cress biomass production per plant was well correlated to the total aromatic hydrocarbon concentration (R-2 = 0.79, n = 6), while cress seed germination was correlated (R-2 = 0.82, n = 6) with total concentration of "highly water-soluble aromatic hydrocarbons" (HSaromatics). The observed ecotoxicity of the leaching water for Microtox-bacteria related well to calculated (based on the HPLC-GCXGC/FID results) petroleum hydrocarbon equilibrium concentrations in water. (C) 2009 Elsevier Ltd. All rights reserved.
引用
收藏
页码：1508 / 1513
页数：6
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