N-arylation of pyrrolidino[3′,4′:1,2][60]fullerene:: Synthesis under solvent-free conditions and electrochemistry of new C60-acceptor dyads

被引：0

作者：

de la Cruz, P

de la Hoz, A ^{[1
]}

Langa, F

Martín, N

Pérez, MC

Sánchez, L

机构：

[1] Univ Castilla La Mancha, Fac Quim, Dept Quim Organ, E-13071 Ciudad Real, Spain

[2] Univ Complutense, Fac Quim, Dept Quim Organ, E-28040 Madrid, Spain

[3] Univ Castilla La Mancha, Fac Ciencias Medio Ambiente, Dept Quim Organ, E-45071 Toledo, Spain

来源：

EUROPEAN JOURNAL OF ORGANIC CHEMISTRY | 1999年 / 1999卷 / 12期

关键词：

cyclic voltammetry; fullerenes; phase-transfer catalysis;

D O I：

10.1002/(SICI)1099-0690(199912)1999:12<3433::AID-EJOC3433>3.0.CO;2-O

中图分类号：

O62 [有机化学];

学科分类号：

070303 ; 081704 ;

摘要：

Several pyrrolidinofullerenes were N-arylated by phase-transfer catalysis in the absence of solvent. The electrochemical behaviour of the novel C-60-acceptor dyads was studied by cyclic voltammetry which showed that the nitro groups on the N-phenyl ring have a strong influence on the reduction potential values. Theoretical calculations at the semiempirical PM3 level fully support the experimental redox potential values.

引用

页码：3433 / 3436

页数：4

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