Strong-field ionization (SFI) has been shown to prepare wave packets with few-femtosecond periods. Here, we explore whether this technique can be extended to the attosecond time scale. We introduce an intuitive model, which is based on the Fourier transform of the subcycle SFI rate, for predicting the bandwidth of ionic states that can be coherently prepared by SFI. The coherent bandwidth decreases considerably with increasing central wavelength of the ionizing pulse but it is much less sensitive to its intensity. Many-body calculations based on time-dependent configuration-interaction singles support these results. The influence of channel interactions and laser-induced dynamics within the ion is discussed. Our results further predict that multicycle femtosecond pulses can coherently prepare subfemtosecond wave packets with higher selectivity and versatility compared to single-cycle pulses with an additional sensitivity to the mutual parity of the prepared states.
机构:
Univ Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, HungaryUniv Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, Hungary
Majorosi, Szilard
Benedict, Mihaly G.
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Univ Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, HungaryUniv Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, Hungary
Benedict, Mihaly G.
Czirjak, Attila
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Univ Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, Hungary
ELI HU Nonprofit Ltd, ELI ALPS, Dugon Ter 13, H-6720 Szeged, HungaryUniv Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, Hungary
机构:
Kansas State Univ, Dept Phys, Manhattan, KS 66506 USA
Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USAKansas State Univ, Dept Phys, Manhattan, KS 66506 USA