Attosecond transient-absorption dynamics of xenon core-excited states in a strong driving field

被引:23
|
作者
Kobayashi, Yuki [1 ]
Timmers, Henry [1 ]
Sabbar, Mazyar [1 ]
Leone, Stephen R. [1 ,2 ,3 ]
Neumark, Daniel M. [1 ,2 ]
机构
[1] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
[2] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA
[3] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
基金
美国国家科学基金会;
关键词
OSCILLATIONS; XE;
D O I
10.1103/PhysRevA.95.031401
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We present attosecond transient-absorption experiments on xenon 4d(-1) 6p core-level states resonantly driven by intense (1.6x10(14)W/cm(2)) few-cycle near-infrared laser pulses. In this strongly driven regime, broad induced absorption features with half-cycle (1.3-fs) delay-dependent modulation are observed over the range of 58-65 eV, predicted as a signature of the breakdown of the rotating-wave approximation in strong-field driving of Autler-Townes splitting [A. N. Pfeiffer and S. R. Leone, Phys. Rev. A 85, 053422 (2012)]. Relevant atomic states are identified by a numerical model involving three electronic states, and the mechanism behind the broad induced absorption is discussed in the Floquet formalism. These results demonstrate that a near-infrared field well into the tunneling regime can still control the optical properties of an atomic system over a several-electron-volt spectral range and with attosecond precision.
引用
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页数:5
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