Molecular Resonance Raman and Rayleigh Scattering Stimulated by a Short Laser Pulse

被引:1
|
作者
Hagedorn, George A. [1 ,2 ]
Valeev, Edward F. [2 ,3 ]
机构
[1] Virginia Polytech Inst & State Univ, Dept Math, Blacksburg, VA 24061 USA
[2] Virginia Polytech Inst & State Univ, Ctr Stat Mech Math Phys & Theoret Chem, Blacksburg, VA 24061 USA
[3] Virginia Polytech Inst & State Univ, Dept Chem, Blacksburg, VA 24061 USA
基金
美国国家科学基金会;
关键词
Rayleigh scattering; Raman scattering; Born-Oppenheimer approximation; SPECTROSCOPY; POTENTIALS; ABSORPTION; RADIATION;
D O I
10.1007/s10955-013-0820-y
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We study a simple model for a molecule subjected to a short laser pulse. We derive very simple expressions for resonance Raman and resonance Rayleigh scattering amplitudes to leading order in the strength mu of the laser and the Born-Oppenheimer parameter I mu for the molecule. We also briefly consider the situation where the incident light is close to, but not exactly at the resonance frequency for an electronic transition of the molecule.
引用
收藏
页码:522 / 542
页数:21
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