Direct visualization of phonon-polariton focusing and amplitude enhancement

被引:10
|
作者
Stoyanov, NS [1 ]
Ward, DW [1 ]
Feurer, T [1 ]
Nelson, KA [1 ]
机构
[1] MIT, Dept Chem, Cambridge, MA 02139 USA
来源
JOURNAL OF CHEMICAL PHYSICS | 2002年 / 117卷 / 06期
关键词
D O I
10.1063/1.1491952
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We report a new method to generate focused phonon polaritons inside ferroelectric crystals. Using an excitation pulse in the form of a ring we generate a phonon-polariton wave packet that propagates inward toward a focal point at the center. This results in a sharp increase in the polariton intensity. It also permits direct visualization and quantitative measurements of the Gouy phase shift and of anisotropy in polariton propagation. Since vibrational and electromagnetic modes are coupled, coherent vibrational amplitudes can be increased substantially through exploitation of electromagnetic wave propagation. (C) 2002 American Institute of Physics.
引用
收藏
页码:2897 / 2901
页数:5
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