Are there localized saddles behind the heterogeneous dynamics of supercooled liquids?

被引:27
|
作者
Coslovich, D.
Pastore, G.
机构
[1] Univ Trieste, Dipartimento Fis Teor, I-34100 Trieste, Italy
[2] CNR INFM Democritos Natl Simulat Ctr, I-34014 Trieste, Italy
来源
EUROPHYSICS LETTERS | 2006年 / 75卷 / 05期
关键词
D O I
10.1209/epl/i2006-10175-8
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We numerically study the interplay between heterogeneous dynamics and properties of negatively curved regions of the potential energy surface in a model glassy system. We find that the unstable modes of saddles and quasi-saddles undergo a localization transition close to the Mode-Coupling critical temperature. We also find evidence of a positive spatial correlation between clusters of particles having large displacements in the unstable modes and dynamical heterogeneities.
引用
收藏
页码:784 / 790
页数:7
相关论文
共 50 条
  • [1] Spatially heterogeneous dynamics in supercooled liquids
    Ediger, MD
    [J]. ANNUAL REVIEW OF PHYSICAL CHEMISTRY, 2000, 51 : 99 - 128
  • [2] Saddles in the energy landscape probed by supercooled liquids
    Angelani, L
    Di Leonardo, R
    Ruocco, G
    Scala, A
    Sciortino, F
    [J]. PHYSICAL REVIEW LETTERS, 2000, 85 (25) : 5356 - 5359
  • [3] Spatially heterogeneous dynamics in supercooled liquids.
    Ediger, MD
    [J]. ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 1998, 215 : U159 - U159
  • [4] Spatially heterogeneous dynamics in deeply supercooled liquids
    Wang, CY
    Ediger, MD
    [J]. SLOW DYNAMICS IN COMPLEX SYSTEMS, 1999, 469 : 339 - 349
  • [5] Heterogeneous relaxation patterns in supercooled liquids studied by solvation dynamics
    Wendt, H
    Richert, R
    [J]. PHYSICAL REVIEW E, 2000, 61 (02): : 1722 - 1728
  • [6] Local Plastic Response and Slow Heterogeneous Dynamics of Supercooled Liquids
    Li, Yan-Wei
    Yao, Yugui
    Ciamarra, Massimo Pica
    [J]. PHYSICAL REVIEW LETTERS, 2022, 128 (25)
  • [7] Heterogeneous relaxation patterns in supercooled liquids studied by solvation dynamics
    Wendt, Hauke
    Richert, Ranko
    [J]. 1722, American Physical Society (61):
  • [8] Molecular dynamics studies of heterogeneous dynamics and dynamic crossover in supercooled atomic liquids
    Andersen, HC
    [J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2005, 102 (19) : 6686 - 6691
  • [9] A theory of localized excitations in supercooled liquids
    Hasyim, Muhammad R.
    Mandadapu, Kranthi K.
    [J]. JOURNAL OF CHEMICAL PHYSICS, 2021, 155 (04):
  • [10] Dominant Effect of Heterogeneous Dynamics on Homogenous Crystal Nucleation in Supercooled Liquids
    Zanotto, Edgar D.
    Montazerian, Maziar
    [J]. FRONTIERS IN PHYSICS, 2020, 8