A study of the transport phenomena in a wall-coated micro steam-methanol reformer

被引:7
|
作者
Lee, Ming-Tsang [1 ]
Grigoropoulos, Costas P. [2 ]
Greif, Ralph [2 ]
机构
[1] Natl Chung Hsing Univ, Dept Mech Engn, Taichung 40227, Taiwan
[2] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA
关键词
Methanol-steam reformer; Microreformer; Wall-coated reformer; PACKED-BED REACTORS; HYDROGEN-PRODUCTION; FUEL-CELLS; CATALYST; PERFORMANCE;
D O I
10.1016/j.ijhydene.2013.11.107
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Microreactors have important advantages due to the increased heat and mass transfer resulting from the small dimensions of the system. This results in enhanced performance and efficiency. Microreformers with wall-coated or suspended catalytic layer configurations have been studied due to their lower transport resistances compared to packed-bed microreformers. In the present work, a theoretical study of the reacting flow in a wall-coated microreformer is carried out. The theoretical results for the conversions and carbon monoxide concentration of wall-coated reformers are compared with the reported experimental data. The effects of important parameters for wall-coated reformers such as the catalyst layer thickness, wall temperature, and the flow velocity of the reactants are studied. Recommendations for the design of micro wall-coated reformers are provided. Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:2008 / 2017
页数:10
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