Investigation of giant magnetoconductance in organic devices based on hopping mechanism

被引:12
|
作者
Yang, F. J. [1 ]
Qin, W. [1 ]
Xie, S. J. [1 ]
机构
[1] Shandong Univ, Sch Phys, State Key Lab Crystal Mat, Jinan 250100, Peoples R China
来源
JOURNAL OF CHEMICAL PHYSICS | 2014年 / 140卷 / 14期
关键词
LIGHT-EMITTING-DIODES; ROOM-TEMPERATURE; SEMICONDUCTING MATERIALS; CONJUGATED POLYMERS; ELECTRON-MOBILITY; MAGNETORESISTANCE; FILMS;
D O I
10.1063/1.4869936
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We suggest a spin-dependent hopping mechanism which includes the effect of the external magnetic field as well as hyperfine interaction (HFI) to explain the observed giant magnetoconductance (MC) in non-magnetic organic devices. Based on the extended Marcus theory, we calculate the MC by using the master equation. It is found that a MC value as large as 91% is obtained under a low driving voltage. For suitable parameters, the theoretical results are in good agreement with the experimental data. Influences of the carrier density, HFI, and the carrier localization on the MC value are investigated. Especially, it is found that a low-dimensional structure of the organic materials is favorable to get a large MC value. (C) 2014 AIP Publishing LLC.
引用
收藏
页数:5
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