Resonant inelastic soft x-ray scattering of CdS: A two-dimensional electronic structure map approach

被引：36

作者：

Weinhardt, L. ^{[1
,2
]}

Fuchs, O. ^{[1
]}

Fleszar, A. ^{[2
]}

Baer, M. ^{[2
]}

Blum, M. ^{[1
,2
]}

Weigand, M. ^{[1
]}

Denlinger, J. D. ^{[3
]}

Yang, W. ^{[3
]}

Hanke, W. ^{[2
]}

Umbach, E. ^{[1
,4
]}

Heske, C. ^{[2
]}

机构：

[1] Univ Wurzburg, D-97074 Wurzburg, Germany

[2] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA

[3] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA

[4] FZ Karlsruhe, D-76344 Eggenstein Leopoldshafen, Germany

来源：

PHYSICAL REVIEW B | 2009年 / 79卷 / 16期

关键词：

band structure; cadmium compounds; density functional theory; fluorescence; II-VI semiconductors; wave functions; X-ray scattering; SOLAR-CELL HETEROJUNCTION; BAND-STRUCTURE; FLUORESCENCE; NANOCRYSTALS; LUMINESCENCE; ABSORPTION; SPECTRA; SOLIDS; ZNS;

D O I：

10.1103/PhysRevB.79.165305

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

Resonant inelastic x-ray scattering (RIXS) with soft x rays is uniquely suited to study the electronic structure of a variety of materials, but is currently limited by low (fluorescence yield) count rates. This limitation is overcome with a high-transmission spectrometer that allows to measure soft x-ray RIXS "maps." The S L(2,3) RIXS map of CdS is discussed and compared with density-functional calculations. The map allows the extraction of decay channel-specific "absorption spectra" giving detailed insight into the wave functions of occupied and unoccupied electronic states.

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页数：5

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