Ag-modified ultrathin Bi12O17Cl2 nanosheets: photo-assisted Ag exfoliation synthesis and enhanced photocatalytic performance

被引：53

作者：

Wang, Yaozhu ^{[1
]}

Huang, Xueyan ^{[1
]}

Wang, Kaiqiang ^{[1
]}

Zhang, Lulu ^{[1
]}

Wang, Bo ^{[1
]}

Fang, Zhibin ^{[1
]}

Zhao, Yan ^{[1
]}

Gao, Fan ^{[1
]}

Liu, Ping ^{[1
]}

Feng, Wenhui ^{[2
]}

机构：

[1] Fuzhou Univ, Res Inst Photocatalysis, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350116, Fujian, Peoples R China

[2] Changsha Univ, Hunan Prov Collaborat Innovat Ctr Environm & Ener, Changsha 410022, Hunan, Peoples R China

来源：

JOURNAL OF MATERIALS CHEMISTRY A | 2018年 / 6卷 / 19期

基金：

中国国家自然科学基金; 国家科技攻关计划;

关键词：

GRAPHITIC CARBON NITRIDE; VISIBLE-LIGHT; HYDROGEN GENERATION; SCALABLE PRODUCTION; CO2; REDUCTION; GRAPHENE; EFFICIENT; METHANOL; LAYERS; MOS2;

D O I：

10.1039/c8ta01403e

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Ultrathin Bi12O17Cl2 nanosheets, with the thickness of 3-4 nm, were prepared by the photo-assisted Ag exfoliation method. This method not only achieves the thickness regulation, but also introduces elemental silver on the surfaces of ultrathin Bi12O17Cl2 nanosheets. The obtained ultrathin Bi12O17Cl2 nanosheets modified with Ag show enhanced visible light absorption, improved carrier generation and separation efficiency under visible light irradiation. Their photocatalytic performance for rhodamine B (RhB) degradation is 5 times higher than that of bulk Bi12O17Cl2. It is expected that the present synthetic strategy may provide a new design concept for the fabrication of ultrathin structures.

引用

页码：9200 / 9208

页数：9

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