Influence of spectral diffusion on single-molecule photon statistics

被引：49
|
作者：
He, Y [1 ]
Barkai, E [1 ]
机构：
[1] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA
来源：
PHYSICAL REVIEW LETTERS | 2004年 / 93卷 / 06期
基金：
美国国家科学基金会;
关键词：
D O I：
10.1103/PhysRevLett.93.068302
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
We investigate the distribution of the number of photons emitted by a single molecule undergoing a spectral diffusion process and interacting with a continuous wave field. Using a generating function formalism an exact analytical formula for Mandel's Q parameter is obtained. The solution, which is valid for weak and strong excitation fields, exhibits transitions between (i) quantum sub-Poissonian and classical super-Poissonian behaviors, and (ii) fast to slow modulation limits.
引用
收藏
页码：068302 / 1
页数：4
相关论文
共 50 条
  • [41] Single-molecule spectral fluctuations at room temperature
    H. Peter Lu
    X. Sunney Xie
    Nature, 1997, 385 : 143 - 146
  • [42] Intramolecular Distances and Dynamics from the Combined Photon Statistics of Single-Molecule FRET and Photoinduced Electron Transfer
    Haenni, Dominik
    Zosel, Franziska
    Reymond, Luc
    Nettels, Daniel
    Schuler, Benjamin
    JOURNAL OF PHYSICAL CHEMISTRY B, 2013, 117 (42): : 13015 - 13028
  • [43] Full counting statistics of a single-molecule quantum dot
    Dong, Bing
    Ding, G. H.
    Lei, X. L.
    PHYSICAL REVIEW B, 2013, 88 (07)
  • [44] Tunable electron counting statistics in a single-molecule magnet
    Xue, Hai-Bin
    Nie, Y. -H.
    Li, Z. -J.
    Liang, J. -Q.
    JOURNAL OF APPLIED PHYSICS, 2010, 108 (03)
  • [45] Slow Single-Molecule Diffusion in Liquid Crystals
    Pumpa, Martin
    Cichos, Frank
    JOURNAL OF PHYSICAL CHEMISTRY B, 2012, 116 (49): : 14487 - 14493
  • [46] Visualizing single-molecule diffusion in mesoporous materials
    Andreas Zürner
    Johanna Kirstein
    Markus Döblinger
    Christoph Bräuchle
    Thomas Bein
    Nature, 2007, 450 : 705 - 708
  • [47] Single-Molecule Tracking of Polymer Surface Diffusion
    Skaug, Michael J.
    Mabry, Joshua N.
    Schwartz, Daniel K.
    JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2014, 136 (04) : 1327 - 1332
  • [48] Single-molecule FRET with diffusion and conformational dynamics
    Gopich, Irina V.
    Szabo, Attila
    JOURNAL OF PHYSICAL CHEMISTRY B, 2007, 111 (44): : 12925 - 12932
  • [49] Single-molecule tracking of polymer surface diffusion
    20140617290006
    Schwartz, D.K. (daniel.schwartz@colorado.edu), 1600, American Chemical Society (136):
  • [50] Visualizing single-molecule diffusion in mesoporous materials
    Zuerner, Andreas
    Kirstein, Johanna
    Doeblinger, Markus
    Braeuchle, Christoph
    Bein, Thomas
    NATURE, 2007, 450 (7170) : 705 - +
12345