Off-resonant double-resonance optical-pumping spectra and their application in a multiphoton cesium magneto-optical trap

We present an investigation of double-resonance optical pumping ( DROP) spectra under the condition of single-photon frequency detuning based on a cesium 6S(1/2)- 6P(3/2)- 8S(1/2) ladder-type system with a room-temperature vapor cell. Two DROP peaks are found, and their origins are explored. One peak has a narrow linewidth due to the atomic coherence for a counterpropagating configuration; the other peak has a broad linewidth, owing to the spontaneous decay for a copropagating configuration. This kind of off-resonant DROP spectrum can be used to control and offset-lock a laser frequency to a transition between excited states. We apply this technique to a multiphoton cesium magneto-optical trap, which can efficiently trap atoms on both red and blue sides of the two-photon resonance.