Template-directed synthesis of mechanically interlocked molecular bundles using dynamic covalent chemistry

被引：79
|
作者：
Northrop, Brian H.
Arico, Fabio
Tangchiavang, Nick
Badjic, Jovica D.
Stoddart, J. Fraser
机构：
[1] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA
[2] Univ Calif Los Angeles, Calif NanoSyst Inst, Los Angeles, CA 90095 USA
来源：
ORGANIC LETTERS | 2006年 / 8卷 / 18期
关键词：
D O I：
10.1021/ol061262u
中图分类号：
O62 [有机化学];
学科分类号：
070303 ; 081704 ;
摘要：
Mixing the dipyrido[24] crown-8 derivatives carrying one or two formyl group(s) on the 4 position(s) of their pyridine ring(s) with a 3symmetrical trisammonium ion template in a 3: 1 ratio in CD3NO2 results in the formation of thermodynamically stable [4] which, upon addition of a 1,3,5-trisaminobenzene cap, form mechanically interlocked molecular bundles with one and two caps, by virtue of dynamic imine bond formation.
引用
收藏
页码：3899 / 3902
页数：4
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