Template-directed synthesis of mechanically interlocked molecular bundles using dynamic covalent chemistry

被引：79
|
作者：
Northrop, Brian H.
Arico, Fabio
Tangchiavang, Nick
Badjic, Jovica D.
Stoddart, J. Fraser
机构：
[1] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA
[2] Univ Calif Los Angeles, Calif NanoSyst Inst, Los Angeles, CA 90095 USA
来源：
ORGANIC LETTERS | 2006年 / 8卷 / 18期
关键词：
D O I：
10.1021/ol061262u
中图分类号：
O62 [有机化学];
学科分类号：
070303 ; 081704 ;
摘要：
Mixing the dipyrido[24] crown-8 derivatives carrying one or two formyl group(s) on the 4 position(s) of their pyridine ring(s) with a 3symmetrical trisammonium ion template in a 3: 1 ratio in CD3NO2 results in the formation of thermodynamically stable [4] which, upon addition of a 1,3,5-trisaminobenzene cap, form mechanically interlocked molecular bundles with one and two caps, by virtue of dynamic imine bond formation.
引用
收藏
页码：3899 / 3902
页数：4
相关论文
共 50 条
  • [1] Template-directed dynamic synthesis of mechanically interlocked dendrimers
    Leung, KCF
    Aricó, F
    Cantrill, SJ
    Stoddart, JF
    JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (16) : 5808 - 5810
  • [2] Template-directed dynamic synthesis of mechanically interlocked dendrimers
    Stoddart, JF
    Leung, KCF
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2005, 230 : U4118 - U4119
  • [3] Efficient routes to novel molecular architectures - Template-directed synthesis of mechanically interlocked suitanes
    Northrop, Brian H.
    Spruell, Jason M.
    Stoddart, J. Frasier
    CHIMICA OGGI-CHEMISTRY TODAY, 2007, 25 (03) : 4 - 7
  • [4] Template-directed synthesis of multiply mechanically interlocked molecules under thermodynamic control
    Aricó, F
    Chang, T
    Cantrill, SJ
    Khan, SI
    Stoddart, JF
    CHEMISTRY-A EUROPEAN JOURNAL, 2005, 11 (16) : 4655 - 4666
  • [5] Template-directed dynamic combinatorial chemistry
    Stefankiewicz, Artur R.
    Sambrook, Mark
    Sanders, Jeremy K. M.
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2012, 244
  • [6] Sequence information transfer using covalent template-directed synthesis
    Nunez-Villanueva, Diego
    Ciaccia, Maria
    Iadevaia, Giulia
    Sanna, Elena
    Hunter, Christopher A.
    CHEMICAL SCIENCE, 2019, 10 (20) : 5258 - 5266
  • [7] Dynamic Covalent Chemistry for Synthesis and Co-conformational Control of Mechanically Interlocked Molecules
    Yu, Jingjing
    Gaedke, Marius
    Schaufelberger, Fredrik
    EUROPEAN JOURNAL OF ORGANIC CHEMISTRY, 2023, 26 (08)
  • [8] Capping Strategies for Covalent Template-Directed Synthesis of Linear Oligomers Using CuAAC
    Ciaccia, Maria
    Nunez-Villanueva, Diego
    Hunter, Christopher A.
    JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2019, 141 (27) : 10862 - 10875
  • [9] Template-Directed Synthesis of Molecular Nanorings and Cages
    Bols, Pernille S.
    Anderson, Harry L.
    ACCOUNTS OF CHEMICAL RESEARCH, 2018, 51 (09) : 2083 - 2092
  • [10] Template-directed synthesis and supramolecular chemistry of porphyrin nanorings
    Anderson, Harry L.
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2014, 247
12345