Electron emission and fragmentation of C60 in collisions with energetic particles

被引:2
|
作者
Itoh, A [1 ]
Majima, T [1 ]
机构
[1] Kyoto Univ, Quantum Sci & Engn Ctr, Kyoto 6068501, Japan
关键词
C-60; fullererene; collision; ionization; fragmentation; cluster;
D O I
10.1016/j.vacuum.2003.12.035
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have studied ionization and fragmentation of C-60 induced in collisions with fast helium, silicon and gold ions. Fragment ions and electrons produced were measured simultaneously in coincidence with outgoing charge-selected projectile ions. By means of this triple coincidence method we obtained successfully detailed information about the correlated emission process between electrons and fragment ions. It was found that the number of emitted electrons n(e) depends strongly on. the cluster size of fragment ions and ne increases with decreasing cluster size. Also, we found that, with increasing atomic number of the projectile ions, the C-60-multi-fragmentation becomes more prominent and the value of n(e) increases as well, indicating clearly the importance of electronic excitation effects. As a more important new result, it was found that the multi-fragmentation is induced rather strongly even in such collisions where only a few electrons are emitted. It is safely concluded that the accompanying internal excitation plays an essential role in the C-60-multi-fragmentation. (C) 2004 Elsevier Ltd. All rights reserved.
引用
收藏
页码:53 / 58
页数:6
相关论文
共 50 条
  • [41] Excitation of C60 by electron impact
    Gordeev, YS
    Mikoushkin, VM
    Shnitov, VV
    MOLECULAR MATERIALS, 2000, 13 (1-4): : 1 - 12
  • [42] On the nature of electron correlation in C60
    Stueck, David
    Baker, Thomas A.
    Zimmerman, Paul
    Kurlancheek, Westin
    Head-Gordon, Martin
    JOURNAL OF CHEMICAL PHYSICS, 2011, 135 (19):
  • [43] Atomic collisions involving C60 and collective excitation
    Tribedi, L. C.
    Kelkar, A. H.
    INDIAN JOURNAL OF PHYSICS, 2011, 85 (12) : 1749 - 1760
  • [44] Atomic collisions involving C60 and collective excitation
    L. C. Tribedi
    A. H. Kelkar
    Indian Journal of Physics, 2011, 85 : 1749 - 1760
  • [45] Thermionic emission and fragmentation of C-60
    Hansen, K
    Echt, O
    PHYSICAL REVIEW LETTERS, 1997, 78 (12) : 2337 - 2340
  • [46] Electron capture and energy loss in ∼100 keV collisions of atomic and molecular ions on C60
    Larsson, MO
    Hvelplund, P
    Larsen, MC
    Shen, H
    Cederquist, H
    Schmidt, HT
    INTERNATIONAL JOURNAL OF MASS SPECTROMETRY, 1998, 177 (01) : 51 - 62
  • [47] High electron stabilization rate in slow collisions of bare Ne10+ with C60
    J. Bernard
    R. Brédy
    L. Chen
    S. Martin
    A. Salmoun
    M.-C. Buchet-Poulizac
    B. Wei
    The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics, 2005, 33 : 229 - 234
  • [48] High electron stabilization rate in slow collisions of bare Ne10+ with C60
    Bernard, J
    Brédy, R
    Chen, L
    Martin, S
    Salmoun, A
    Buchet-Poulizac, MC
    Wei, B
    EUROPEAN PHYSICAL JOURNAL D, 2005, 33 (02): : 229 - 234
  • [49] Electron transfer and multi-ionization in slow collisions Of C60 with highly charged ions
    Wei, B
    Ma, X
    Zhu, XL
    Liu, HP
    Wang, ZL
    Sha, S
    Feng, WT
    Cao, SP
    Qian, DB
    Li, B
    Chen, LF
    NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 2005, 235 : 378 - 381
  • [50] Efficiency of thermionic emission from C60
    Deng, RP
    Echt, O
    JOURNAL OF PHYSICAL CHEMISTRY A, 1998, 102 (15): : 2533 - 2539