A novel high-stability Au(III)/Schiff-based catalyst for acetylene hydrochlorination reaction

被引：46

作者：

Huang, Chaofeng ^{[1
]}

Zhu, Mingyuan ^{[1
,2
]}

Kang, Lihua ^{[1
,2
]}

Dai, Bin ^{[1
,2
]}

机构：

[1] Shihezi Univ, Sch Chem & Chem Engn, Shihezi 832000, Xinjiang, Peoples R China

[2] Key Lab Green Proc Chem Engn Xinjiang Bingtuan, Shihezi 832000, Xinjiang, Peoples R China

来源：

CATALYSIS COMMUNICATIONS | 2014年 / 54卷

基金：

中国国家自然科学基金;

关键词：

AuCl2(phen)]Cl; Acetylene hydrochlorination;

D O I：

10.1016/j.catcom.2014.05.024

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Herein, we reported on the application of an Au(III)/Schiff-based catalyst in acetylene hydrochlorination reaction. The [AuCl2(phen)]Cl catalyst exhibited excellent stability, and acetylene conversion was maintained at >90% after 40 h of operation. The excellent stability of the [AuCl2(phen)]Cl catalyst was attributed to the presence of the 1,10-phenanthroline ligand that partially inhibited the reduction of the Au3+ active component. (C) 2014 Elsevier B.V. All rights reserved.

引用

页码：61 / 65

页数：5

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