Concentrations of trace elements and PCDD/Fs around a municipal solid waste incinerator in Girona (Catalonia, Spain). Human health risks for the population living in the neighborhood

被引:38
|
作者
Rovira, Joaquim [1 ,2 ]
Nadal, Marti [1 ]
Schuhmacher, Marta [1 ,2 ]
Domingo, Jose L. [1 ]
机构
[1] Univ Rovira & Virgili, IISPV, Sch Med, Lab Toxicol & Environm Hlth, St Llorenc 21, Reus 43201, Catalonia, Spain
[2] Univ Rovira & Virgili, Dept Engn Quim, Environm Engn Lab, Av Paisos Catalans 26, E-43007 Tarragona, Catalonia, Spain
关键词
Trace elements; Dioxins and furans; Soil; Air; MSWI; Back-trajectories; Risk assessment; DIBENZO-P-DIOXINS; TEMPORAL TRENDS; AMBIENT AIR; ENVIRONMENTAL SURVEILLANCE; VEGETATION SAMPLES; HEAVY-METALS; LONG-TERM; VICINITY; SOIL; PLANT;
D O I
10.1016/j.scitotenv.2018.02.175
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Previously to the modernization of the municipal solid waste incinerator (MSWI) of Campdora (Girona, Catalonia, Spain) two sampling campaigns (2015 and 2016) were conducted. In each campaign, 8 soil and 4 air samples (PM10 and total particle phase and gas phase) were collected. The levels of As, Cd, Co, Cr, Cu, Hg, Mn, Ni, Pb, Sb, Sn, Tl and V, and PCDD/Fswere analysed at different distances and wind directions around the MSWI. Environmental levels of trace elements and PCDD/Fs were used to assess exposure and health risks (carcinogenic and non-carcinogenic) for the population living around the facility. In soils, no significant differences were observed for trace elements and PCDD/Fs between both campaigns. In air, significant higher levels of As, Cd, Co, Mn, Ni, Pb, Tl and V were detected in 2016. Regarding soil levels, only Cd (distances) and As, Cu, Mn, and Ni (wind directions) showed significant differences. No differences were noted in the concentrations of trace elements and PCDD/Fs in air levels with respect to distances and directions to the MSWI. No differences were registered in air levels (elements and PCDD/Fs) between points influenced by MSWI emissions and background point. However some differences in congener profile were noted regarding from where back-trajectories come from (HYSPLIT model results), pointing some influence of Barcelona metropolitan area. The concentrations of trace elements and PCDD/Fs were similar -or even lower-than those reported around other MSWIs in Catalonia and various countries. Non-carcinogenic risks were below the safety limit (HQ < 1). In turn, carcinogenic risks due to exposure to trace elements and PCDD/Fs were in acceptable ranges, according to national and international standard regulations. (C) 2018 Elsevier B.V. All rights reserved.
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页码:34 / 45
页数:12
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