Signature of Kondo hybridisation with an orbital-selective Mott phase in 4d Ca2-xSrxRuO4

被引：12

作者：

Kim, Minsoo ^{[1
,2
]}

Kwon, Junyoung ^{[1
,2
]}

Kim, Choong H. ^{[1
,2
]}

Kim, Younsik ^{[1
,2
]}

Chung, Daun ^{[3
]}

Ryu, Hanyoung ^{[1
,2
]}

Jung, Jongkeun ^{[1
,2
]}

Kim, Beom Seo ^{[1
,2
]}

Song, Dongjoon ^{[1
,2
]}

Denlinger, Jonathan D. ^{[4
]}

Han, Moonsup ^{[5
]}

Yoshida, Yoshiyuki ^{[6
]}

Mizokawa, Takashi ^{[7
]}

Kyung, Wonshik ^{[1
,2
]}

Kim, Changyoung ^{[1
,2
]}

机构：

[1] Inst Basic Sci IBS, Ctr Correlated Electron Syst, Seoul 08826, South Korea

[2] Seoul Natl Univ, Dept Phys & Astron, Seoul 08826, South Korea

[3] Seoul Natl Univ, Coll Liberal Studies, Seoul 08826, South Korea

[4] Lawrence Berkeley Natl Lab, Adv Light Source ALS, Berkeley, CA 94720 USA

[5] Univ Seoul, Dept Phys, Seoul 02504, South Korea

[6] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan

[7] Waseda Univ, Dept Appl Phys, Tokyo 1698555, Japan

来源：

NPJ QUANTUM MATERIALS | 2022年 / 7卷 / 01期

关键词：

LOW-ENERGY-SCALE; TRANSITION;

D O I：

10.1038/s41535-022-00471-5

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

The heavy fermion state with Kondo-hybridisation (KH), usually manifested in f-electron systems with lanthanide or actinide elements, was recently discovered in several 3d transition metal compounds without f-electrons. However, KH has not yet been observed in 4d/5d transition metal compounds, since more extended 4d/5d orbitals do not usually form flat bands that supply localised electrons appropriate for Kondo pairing. Here, we report a substitution- and temperature-dependent angle-resolved photoemission study on 4d Ca2-xSrxRuO4, which shows the signature of KH. We observed a spectral weight transfer in the gamma-band, reminiscent of an orbital-selective Mott phase (OSMP). The Mott localised gamma-band induces the KH with an itinerant beta-band, resulting in spectral weight suppression around the Fermi level. Our work demonstrates the evolution of the OSMP with possible KH among 4d electrons, and thereby expands the material boundary of Kondo physics to 4d multi-orbital systems.

引用

页数：7

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