In this work the strong electromagnetic field of femtosecond Ti:Sa lasers was used to excite surface plasmon oscillations (SPOs) in gold films at room temperature in the Kretschmann geometry. Experimental investigations were carried out using a surface plasmon near field scanning tunneling microscope, measuring its response to excitation at SPO hot spots on the gold surface. Furthermore, the spectra of photoelectrons, liberated by multiplasmon absorption, have also been measured by a time-of-flight spectrometer. In both cases new type of anomalies in both the STM and electron TOF signals have been measured in the same laser intensity range. The existence of these anomalies may be qualitatively understood, by using the intensity-dependent expression for the effective electron-electron scattering potential, derived earlier in a different context. In this theoretical work an effective attraction potential has been predicted in the presence of strong inhomogeneous radiation fields. Copyright (C) EPLA, 2014
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Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
Kim, Youngsang
Creel, Erin B.
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Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
Creel, Erin B.
Corson, Elizabeth R.
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Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
Corson, Elizabeth R.
McCloskey, Bryan D.
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Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA
Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
McCloskey, Bryan D.
Urban, Jeffrey J.
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Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
Urban, Jeffrey J.
Kostecki, Robert
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Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA