Transient enhancement of high-order harmonic generation in expanding molecules

被引:29
|
作者
Pfeifer, T [1 ]
Walter, D
Gerber, G
Emelin, MY
Ryabikin, MY
Chernobrovtseva, MD
Sergeev, AM
机构
[1] Univ Wurzburg, Inst Phys, D-97074 Wurzburg, Germany
[2] Russian Acad Sci, Inst Appl Phys, Nizhnii Novgorod 603950, Russia
来源
PHYSICAL REVIEW A | 2004年 / 70卷 / 01期
关键词
D O I
10.1103/PhysRevA.70.013805
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
High-order harmonic generation (HHG) is limited by the probability of recombination of the returning electron with the parent ion. We show here that the internuclear distance of simplest diatomic molecules, determining differently delocalized initial electronic states, can be used to enhance the HHG conversion efficiency exceeding the atomic one. We propose an experiment based on a double-pulse pump-drive scheme where a strong transient enhancement of the HHG yield is predicted.
引用
收藏
页码:013805 / 1
页数:5
相关论文
共 50 条
  • [21] Dramatic enhancement of high-order harmonic generation in mixed gases
    Takahashi, Eiji J.
    Kanai, Tsuneto
    Nabekawa, Yasuo
    Midorikawa, Katsumi
    Ishikawa, Kenichi L.
    2007 CONFERENCE ON LASERS & ELECTRO-OPTICS/QUANTUM ELECTRONICS AND LASER SCIENCE CONFERENCE (CLEO/QELS 2007), VOLS 1-5, 2007, : 2757 - +
  • [22] High-order harmonic generation
    Salières, P
    ATOMS, SOLIDS, AND PLASMAS IN SUPER-INTENSE LASER FIELDS, 2001, : 83 - 97
  • [23] Effect of orbital symmetry on high-order harmonic generation from molecules
    Shan, B
    Ghimire, S
    Chang, ZH
    PHYSICAL REVIEW A, 2004, 69 (02): : 4
  • [24] Dynamic orbitals in high-order harmonic generation from CO molecules
    Zhang, Bin
    Yuan, Jianmin
    Zhao, Zengxiu
    PHYSICAL REVIEW A, 2014, 90 (03):
  • [25] High-order harmonic generation in vibrating two-electron molecules
    Chirila, C. C.
    Lein, M.
    CHEMICAL PHYSICS, 2009, 366 (1-3) : 54 - 57
  • [26] Role of ellipticity in high-order harmonic generation by homonuclear diatomic molecules
    Odzak, S.
    Milosevic, D. B.
    PHYSICAL REVIEW A, 2010, 82 (02):
  • [27] Ellipticity dependence of high-order harmonic generation from aligned molecules
    Kanai, Tsuneto
    Minemoto, Shinichirou
    Sakai, Hirofumi
    PHYSICAL REVIEW LETTERS, 2007, 98 (05)
  • [28] Quantitative rescattering theory for high-order harmonic generation from molecules
    Le, Anh-Thu
    Lucchese, R. R.
    Tonzani, S.
    Morishita, T.
    Lin, C. D.
    PHYSICAL REVIEW A, 2009, 80 (01)
  • [29] Circular dichroism in high-order harmonic generation from chiral molecules
    Harada, Yoichi
    Haraguchi, Eisuke
    Kaneshima, Keisuke
    Sekikawa, Taro
    PHYSICAL REVIEW A, 2018, 98 (02)
  • [30] Tracing the structure of asymmetric molecules from high-order harmonic generation
    Chen, Yanjun
    Zhang, Bing
    PHYSICAL REVIEW A, 2011, 84 (05):