Source apportionment of particulate matter based on numerical simulation during a severe pollution period in Tangshan, North China

被引:21
|
作者
He, Jianjun [1 ,2 ,3 ]
Zhang, Lei [1 ,2 ]
Yao, Zhanyu [4 ,5 ]
Che, Huizheng [1 ,2 ]
Gong, Sunling [1 ,2 ]
Wang, Min [6 ]
Zhao, Mengxue [6 ]
Jing, Boyu [3 ]
机构
[1] Chinese Acad Meteorol Sci, State Key Lab Severe Weather, Beijing 100081, Peoples R China
[2] Chinese Acad Meteorol Sci, Key Lab Atmospher Chem CMA, Beijing 100081, Peoples R China
[3] State Environm Protect Key Lab Odor Pollut Contro, Tianjin 300071, Peoples R China
[4] Chinese Acad Meteorol Sci, Key Lab Cloud Phys CMA, Beijing 100081, Peoples R China
[5] Chinese Acad Meteorol Sci, State Key Lab Severe Weather, Beijing 100081, Peoples R China
[6] Minist Ecol & Environm Peoples Republ China, Policy Res Ctr Environm & Econ, Beijing 100029, Peoples R China
基金
中国国家自然科学基金;
关键词
Source apportionment; WRF-Chem; FLEXPART; Potential source region; AIR-QUALITY MODEL; METEOROLOGICAL CONDITIONS; SENSITIVITY-ANALYSIS; HAZE EPISODE; AEROSOL; POLLUTANTS; EMISSION; WINTER; PM2.5; IMPLEMENTATION;
D O I
10.1016/j.envpol.2020.115133
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Facing serious air pollution problems, the Chinese government has taken numerous measures to prevent and control air pollution. Understanding the sources of pollutants is crucial to the prevention of air pollution. Using numerical simulation method, this study analysed the contributions of the total local emissions and local emissions from different sectors (such as industrial, traffic, resident, agricultural, and power plant emissions) to PM2.5 concentration, backward trajectory, and potential source regions in Tangshan, a typical heavy industrial city in north China. The impact of multi-scale meteorological conditions on source apportionment was investigated. From October 2016 to March 2017, total local emissions accounted for 46.0% of the near-surface PM2.5 concentration. In terms of emissions from different sectors, local industrial emissions which accounted for 23.1% of the near-surface PM2.5 concentration in Tangshan, were the most important pollutant source. Agricultural emissions were the second most important source, accounting for 10.3% of the near-surface PM2.5 concentration. The contributions of emissions from power plants, traffic, residential sources were 2.0%, 3.0%, and 7.2%, respectively. The contributions of total local emissions and emissions from different sectors depended on multi-scale meteorological conditions, and static weather significantly enhanced the contribution of regional transport to the near-surface PM2.5 concentration. Eight cluster backward trajectories were identified for Tangshan. The PM2.5 concentration for the 8 cluster trajectories significantly differed. The near-surface PM2.5 in urban Tangshan (receptor point) was mainly from the local emissions, and another important potential source regionwas Tianjin. The results of the source apportionment suggested the importance of joint prevention and control of air pollution in some areas where cities or industrial regions are densely distributed. (C) 2020 Elsevier Ltd. All rights reserved.
引用
收藏
页数:13
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