Efficient long-distance energy transport in molecular systems through adiabatic passage

被引:10
|
作者
Dijkstra, Arend G. [1 ,2 ]
Beige, Almut [2 ]
机构
[1] Univ Leeds, Sch Chem, Leeds LS2 9JT, W Yorkshire, England
[2] Univ Leeds, Sch Phys & Astron, Leeds LS2 9JT, W Yorkshire, England
来源
JOURNAL OF CHEMICAL PHYSICS | 2019年 / 151卷 / 03期
基金
英国工程与自然科学研究理事会;
关键词
COHERENCE;
D O I
10.1063/1.5100210
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The efficiencies of light-harvesting complexes in biological systems can be much higher than the current efficiencies of artificial solar cells. In this paper, we therefore propose and analyze an energy transport mechanism which employs adiabatic passages between the states of an artificially designed antenna molecular system to significantly enhance the conversion of incoming light into internal energy. It is shown that the proposed transport mechanism is relatively robust against spontaneous emission and dephasing, while also being able to take advantage of collective effects. Our aim is to provide new insight into the energy transport in molecular complexes and to improve the design of solar cells.
引用
收藏
页数:7
相关论文
共 50 条
  • [21] LONG-DISTANCE TRANSPORT OF EXPORT LAMBS
    KNOWLES, TG
    WARRISS, PD
    BROWN, SN
    KESTIN, SC
    VETERINARY RECORD, 1994, 134 (05) : 107 - 110
  • [22] Long-distance Heat Transport.
    Valasek, Jiri
    Energietechnik Leipzig, 1981, 31 (05): : 186 - 190
  • [23] Long-distance transport of pollen into the Arctic
    Ian D. Campbell
    Karen McDonald
    Michael D. Flannigan
    Joanni Kringayark
    Nature, 1999, 399 : 29 - 30
  • [24] Molecular analysis confirms the long-distance transport of Juniperus ashei pollen
    Mohanty, Rashmi Prava
    Buchheim, Mark Alan
    Anderson, James
    Levetin, Estelle
    PLOS ONE, 2017, 12 (03):
  • [25] LONG-DISTANCE TRANSPORT OF THE CRITICALLY ILL
    RUNCIE, CJ
    TELFER, ABM
    ANAESTHESIA, 1991, 46 (09) : 800 - 801
  • [26] PROTECTING PERISHABLES IN LONG-DISTANCE TRANSPORT
    RATH, E
    AGRICULTURAL ENGINEERING, 1975, 56 (04): : 30 - &
  • [27] LONG-DISTANCE TRANSPORT OF ASSIMILATES IN LAMINARIALES
    SCHMITZ, K
    JOURNAL OF PHYCOLOGY, 1977, 13 : 61 - 61
  • [28] Long-distance spin transport through a graphene quantum Hall antiferromagnet
    Petr Stepanov
    Shi Che
    Dmitry Shcherbakov
    Jiawei Yang
    Ruoyu Chen
    Kevin Thilahar
    Greyson Voigt
    Marc W. Bockrath
    Dmitry Smirnov
    Kenji Watanabe
    Takashi Taniguchi
    Roger K. Lake
    Yafis Barlas
    Allan H. MacDonald
    Chun Ning Lau
    Nature Physics, 2018, 14 : 907 - 911
  • [29] THE MYTH OF LONG-DISTANCE MEGALITH TRANSPORT
    THORPE, RS
    WILLIAMSTHORPE, O
    ANTIQUITY, 1991, 65 (246) : 64 - 73
  • [30] LONG-DISTANCE HEAT-TRANSPORT
    VALASEK, J
    ENERGIETECHNIK, 1981, 31 (05): : 186 - 190