We develop a theory for a type of disorder in condensed matter systems arising from local twist-angle fluctuations in two strongly coupled van der Waals monolayers twisted with respect to each other to create a flat-band moire superlattice. The paradigm of "twist-angle disorder" arises from the currently ongoing intense research activity in the physics of twisted bilayer graphene. In experimental samples of pristine twisted bilayer graphene, which are nominally free of impurities and defects, the main source of disorder is believed to arise from the unavoidable and uncontrollable nonuniformity of the twist angle across the sample. To address this physics of twist-angle disorder, we develop a real-space, microscopic model of twisted bilayer graphene where the angle enters as a free parameter. In particular, we focus on the size of single-particle energy gaps separating the miniband from the rest of the spectrum, the Van Hove peaks, the renormalized Dirac cone velocity near charge neutrality, and the minibandwidth. We find that the energy gaps and minibandwidth are strongly affected by disorder while the renormalized velocity remains virtually unchanged. We discuss the implications of our results for the ongoing experiments on twisted bilayer graphene. Our theory is readily generalized to future studies of twist-angle disorder effects on all electronic properties of moire superlattices created by twisting two coupled van der Waals materials with respect to each other.
机构:
Univ Illinois Urbana & Champaign, Dept Mech Sci & Engn, Urbana, IL 61801 USA
Univ Illinois, Mat Res Lab, Urbana, IL 61801 USAUniv Illinois Urbana & Champaign, Dept Mech Sci & Engn, Urbana, IL 61801 USA
Rakib, Tawfiqur
Pochet, Pascal
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Univ Grenoble Alpes, IriG, Dept Phys, F-38000 Grenoble, France
CEA, Grenoble, FranceUniv Illinois Urbana & Champaign, Dept Mech Sci & Engn, Urbana, IL 61801 USA
Pochet, Pascal
Ertekin, Elif
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Univ Illinois Urbana & Champaign, Dept Mech Sci & Engn, Urbana, IL 61801 USA
Univ Illinois, Mat Res Lab, Urbana, IL 61801 USAUniv Illinois Urbana & Champaign, Dept Mech Sci & Engn, Urbana, IL 61801 USA
Ertekin, Elif
Johnson, Harley T.
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Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USAUniv Illinois Urbana & Champaign, Dept Mech Sci & Engn, Urbana, IL 61801 USA
机构:
Peking Univ, Int Ctr Quantum Mat, Sch Phys, Beijing 100871, Peoples R ChinaPeking Univ, Int Ctr Quantum Mat, Sch Phys, Beijing 100871, Peoples R China
Zhou, Geng-Dong
Wang, Yi-Jie
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Peking Univ, Int Ctr Quantum Mat, Sch Phys, Beijing 100871, Peoples R ChinaPeking Univ, Int Ctr Quantum Mat, Sch Phys, Beijing 100871, Peoples R China
Wang, Yi-Jie
Tong, Ninghua
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Renmin Univ China, Dept Phys, Beijing 100872, Peoples R ChinaPeking Univ, Int Ctr Quantum Mat, Sch Phys, Beijing 100871, Peoples R China
Tong, Ninghua
Song, Zhi-Da
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Peking Univ, Int Ctr Quantum Mat, Sch Phys, Beijing 100871, Peoples R China
Hefei Natl Lab, Hefei 230088, Peoples R China
Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R ChinaPeking Univ, Int Ctr Quantum Mat, Sch Phys, Beijing 100871, Peoples R China
机构:
Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USAUniv Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA
Dai, Shuyang
Xiang, Yang
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Hong Kong Univ Sci & Technol, Dept Math, Hong Kong, Hong Kong, Peoples R ChinaUniv Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA
Xiang, Yang
Srolovitz, David J.
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Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA
Univ Penn, Dept Mech Engn & Appl Mech, Philadelphia, PA 19104 USAUniv Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA