In-situ Photosynthetic Route to Tailor Point Defects in TiO2(B) Nanosheets for Visible Light-Driven Photocatalytic Hydrogen Production

被引:9
|
作者
Wang, Ping [1 ]
Yi, Zhouxiang [1 ]
Zhang, Jiajia [1 ]
Cai, Zhengyang [1 ]
Lyu, Bowen [1 ]
Yang, Junhe [1 ]
Wang, Xianying [1 ]
机构
[1] Univ Shanghai Sci & Technol, Sch Mat Sci & Technol, Jungong Rd 516, Shanghai 200093, Peoples R China
基金
中国国家自然科学基金;
关键词
Photocatalysis; Water splitting; Titanium; Point defects; HIGHLY EFFICIENT; WATER; OXIDE; TI3+; COCATALYSTS; COMPOSITE;
D O I
10.1002/cctc.201900713
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In-situ UV-irradiation activation leads to an intense visible-light absorption of up to 700 nm in ethylene glycolate-stabilized TiO2(B) nanosheets. It is ascribed that the creation of abundant subsurface/lattice oxygen vacancies and Ti3+ centers, along with UV-induced breakdown of Ti-O bonds between ethylene glycolate and TiO2(B). Consequently, the enhanced and stable visible-light-driven photocatalytic H-2 evolution is obtained on defect-rich TiO2(B) nanosheets.
引用
收藏
页码:4252 / 4255
页数:4
相关论文
共 50 条
  • [41] A heterostructure BiOCl nanosheets/TiO2 hollow-tubes composite for visible light-driven efficient photodegradation antibiotic
    Bao, Sarenqiqige
    Liang, Haiou
    Li, Chunping
    Bai, Jie
    JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 2020, 397
  • [42] NiS/Pt loaded on electrospun TiO2 nanofiber with enhanced visible-light-driven photocatalytic hydrogen production br
    Chang, Yu-Cheng
    Zeng, Cheng-Jyun
    Chen, Chin-Yi
    Tsay, Chien-Yie
    Lee, Gang-Juan
    Wu, Jerry J.
    MATERIALS RESEARCH BULLETIN, 2023, 157
  • [43] Highly effective ruthenium-doped TiO2 nanoparticles photocatalyst for visible-light-driven photocatalytic hydrogen production
    Ismael, Mohammed
    NEW JOURNAL OF CHEMISTRY, 2019, 43 (24) : 9596 - 9605
  • [44] Hyperbranched Conjugated Polymer Dots: The Enhanced Photocatalytic Activity for Visible Light-Driven Hydrogen Production
    Zhao, Peng
    Wang, Lijie
    Wu, Yusen
    Yang, Tao
    Ding, Yun
    Yang, Hua Gui
    Hu, Aiguo
    MACROMOLECULES, 2019, 52 (11) : 4376 - 4384
  • [45] AgBr/Polyoxometalate/Graphene Oxide Ternary Composites for Visible Light-Driven Photocatalytic Hydrogen Production
    Gao, Xiaoru
    Wang, Jinfeng
    Xue, Qihui
    Ma, Yuan-Yuan
    Gao, Yuanzhe
    ACS APPLIED NANO MATERIALS, 2021, 4 (02) : 2126 - 2135
  • [46] Nickel oxide/Au porous nanobelts: Synthesis and visible light-driven photocatalytic hydrogen production
    Qian, Xiao-Bing
    Peng, Wen
    Shao, Yi-Biao
    Huang, Jian-Hua
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2018, 43 (04) : 2160 - 2170
  • [47] Facile route for porous N,S co-doped TiO2 nanoparticles for visible light-driven photocatalysis
    Ouyang, Weimin
    Ji, Yajun
    MICRO & NANO LETTERS, 2020, 15 (08) : 566 - 569
  • [48] Relation between photocatalytic activity and preparation conditions for nitrogen-doped visible light-driven TiO2 photocatalysts
    Joung, Soon-Kil
    Amemiya, Takashi
    Murabayashi, Masayuki
    Itoh, Kiminori
    APPLIED CATALYSIS A-GENERAL, 2006, 312 : 20 - 26
  • [49] Photocatalytic production of hydrogen from water using TiO2 and B/TiO2
    Moon, SC
    Mametsuka, H
    Tabata, S
    Suzuki, E
    CATALYSIS TODAY, 2000, 58 (2-3) : 125 - 132
  • [50] Facile synthesis of N-doped biphasic TiO2 nanoparticles with enhanced visible light-driven photocatalytic performance
    Dey, Kamol
    Vaidya, Sonalika
    Gobetti, Anna
    Ramorino, Giorgio
    Ganguli, Ashok K.
    MATERIALS TODAY COMMUNICATIONS, 2022, 33