Simultaneous production of biocrude oil and recovery of nutrients and metals from human feces via hydrothermal liquefaction

被引:104
|
作者
Lu, Jianwen [1 ]
Zhang, Jiaren [2 ]
Zhu, Zhangbing [1 ]
Zhang, Yuanhui [1 ,3 ]
Zhao, Yu [1 ]
Li, Ruirui [1 ]
Watson, Jamison [3 ]
Li, Baoming [1 ]
Liu, Zhidan [1 ]
机构
[1] China Agr Univ, Key Lab Agr Engn Struct & Environm, Coll Water Resources & Civil Engn, Lab Environm Enhancing Energy,Minist Agr, Beijing 100083, Peoples R China
[2] PetroChina Petrochem Res Inst, Beijing 102206, Peoples R China
[3] Univ Illinois, Dept Agr & Biol Engn, Urbana, IL 61801 USA
基金
比尔及梅琳达.盖茨基金会; 中国国家自然科学基金;
关键词
Human feces; Hydrothermal liquefaction; Biocrude oil; Metal distribution; MACROALGAE ENTEROMORPHA-PROLIFERA; WASTE-WATER TREATMENT; OPERATIONAL PARAMETERS; BIOFUEL PRODUCTION; AQUEOUS-PHASE; ALGAL BIOMASS; HUMAN EXCRETA; MICROALGAE; MANURE; TEMPERATURE;
D O I
10.1016/j.enconman.2016.12.052
中图分类号
O414.1 [热力学];
学科分类号
摘要
Hydrothermal liquefaction (HTL) is a thermochemical process specifically suitable for treating wet wastes. This study investigated its, potential for the production of biocrude oil and the recovery of nutrients and metals from human feces via HTL. Specifically, the effects of temperature (260 degrees C, 300 degrees C, 340 degrees C), retention time (10 min, 30 min, 50 min) and total solid (TS) content (5%, 15%, 25%) were studied. The maximum liquefied fraction was 87.89% and the highest biocrude yield reached 34.44% with a higher heating value of 40.29 MJ/kg. Experimental results showed that 54% of carbon in the human feces was migrated to the biocrude oil while 72% of nitrogen was released to the aqueous phase. In addition, most of heavy and alkaline-earth metal elements in the human feces, including Ca (89%), Mg (81%), Al (88%), Fe (72%) and Zn (94%) were distributed in the solid residue, whereas K (89%) and Na (73%) were mainly dissolved into the aqueous phase. This study demonstrated that the efficient degradation of human waste via HTL without any pretreatment and its potential for the valorization in biocrude oil as well as separated nutrients and metals. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:340 / 346
页数:7
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