Single-mode lasing of CsPbBr3 perovskite NWs enabled by the Vernier effect

被引:31
|
作者
Li, Fangtao [1 ,2 ]
Jiang, Mingming [3 ]
Cheng, Yang [4 ]
Zhang, Yufei [1 ]
Yang, Zheng [1 ]
Peng, Yiyao [1 ]
Ma, Wenda [5 ]
Chen, Qiushuo [1 ]
Wang, Chunfeng [5 ]
Liu, Kaihui [4 ]
Wang, Rongming [2 ]
Lu, Junfeng [3 ]
Pan, Caofeng [1 ,4 ,6 ,7 ]
机构
[1] Chinese Acad Sci, CAS Ctr Excellence Nanosci, Beijing Key Lab Micronano Energy & Sensor, Beijing Inst Nanoenergy & Nanosyst, Beijing 100083, Peoples R China
[2] Univ Sci & Technol Beijing, Adv Innovat Ctr Mat Genome Engn, Beijing Key Lab Magnetophotoelect Composite & Int, Sch Math & Phys, Beijing 100083, Peoples R China
[3] Nanjing Univ Aeronaut & Astronaut, Coll Sci, Nanjing 210016, Peoples R China
[4] Peking Univ, Sch Phys, Collaborat Innovat Ctr Quantum Matter, State Key Lab Mesoscop Phys, Beijing 100871, Peoples R China
[5] Shenzhen Univ, Coll Phys & Optoelect Engn, Shenzhen 518060, Peoples R China
[6] Univ Chinese Acad Sci, Sch Nanosci & Technol, Beijing 100049, Peoples R China
[7] Guangxi Univ, Sch Phys Sci & Technol, Ctr Nanoenergy Res, Nanning 530004, Guangxi, Peoples R China
基金
北京市自然科学基金; 中国国家自然科学基金;
关键词
Bromine compounds - Perovskite - Cesium compounds - Lead compounds - Single crystals - Optoelectronic devices - Ion beams;
D O I
10.1039/d0nr08644d
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Inorganic lead halide perovskite (CsPbX3, X = Cl, Br, I) NWs (NWs) have been employed in lasers due to their intriguing attributes of tunable wavelength, low threshold, superior stability, and easy preparation. However, current CsPbX3 NW lasers usually work in a multi-mode modal, impeding their practical applications in optical communication due to the associated false signaling. In this work, high-performance single-mode lasing has been demonstrated by designing and fabricating coupled cavities in the high-quality single-crystal CsPbBr3 NWs via the focused ion beam (FIB) milling approach. The single-mode laser shows a threshold of 20.1 mu J cm(-2) and a high quality factor of similar to 2800 profiting from the Vernier effect, as demonstrated by the experiments and finite-different time-domain (FDTD) simulations. These results demonstrate the promising potentials of the CsPbX3 NW lasers in optical communication and integrated optoelectronic devices.
引用
收藏
页码:4432 / 4438
页数:7
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