PBAT/MXene monolithic solar vapor generator with high efficiency on seawater evaporation and swage purification

被引:13
|
作者
Zhang, Ruiqi [1 ]
Han, Wenjuan [1 ]
Jiang, Hongjian [1 ]
Wang, Xiaofeng [2 ]
Wang, Bo [1 ]
Liu, Chuntai [3 ]
Shen, Changyu [3 ]
机构
[1] Zhengzhou Univ, Sch Mat Sci & Engn, Zhengzhou 450001, Peoples R China
[2] Natl Ctr Int Res Micronano Molding Technol, Sch Mech & Safety Engn, Zhengzhou 450001, Peoples R China
[3] Zhengzhou Univ, Natl Engn Res Ctr Adv Polymer Proc Technol, Key Lab Mat Proc & Mold, Minist Educ, Zhengzhou 450001, Peoples R China
关键词
Solar-driven interfacial water evaporation; Degradable PBAT monolith; MXene; Synergistic effect; Seawater desalination; Salt resistance; STEAM-GENERATION; AEROGEL;
D O I
10.1016/j.desal.2022.116015
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Solar vapor generator (SVG) is undoubtedly a sustainable water treatment technology and good candidate to resolve the water shortage. However, the non-degradable polymer based SVG will bring extra environmental risk when they are scrapped. Herein, we fabricate a degradable interfacial solar vapor generator (DISVG) using PBAT monolith with hierarchical porous morphology via in-situ polymerization of PDA and dip-coating of MXene. Contributed to the MXene and PDA's synergetic effects, the DISVG demonstrates promising solar absorbance (up to 97.07 %), superhydrophilicity, and high evaporation efficiency. Consequently, the DISVG exhibit a high evaporation rate of 1.87 kg m 2 h 1 with a solar steam efficiency of 86.19 % under 1 sun irradiation. The DISVG shows excellent salt and oil resistance because of its good hydrophilicity. Moreover, the DISVG possesses excellent purification capability that can reject above 99 % ions in seawater and dyes in sewage. This research demonstrates a sustainable strategy for the fabrication of DISVG with environmentally friendly, highly efficient and well reliable solar vapor generators for seawater desalination and sewage purification.
引用
收藏
页数:10
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