Atmospheric composition change - global and regional air quality

被引：612

作者：

Monks, P. S. ^{[1
]}

Granier, C. ^{[2
,3
,4
]}

Fuzzi, S. ^{[5
]}

Stohl, A. ^{[6
]}

Williams, M. L. ^{[7
]}

Akimoto, H. ^{[8
]}

Amann, M. ^{[9
]}

Baklanov, A. ^{[10
]}

Baltensperger, U. ^{[11
]}

Bey, I. ^{[12
]}

Blake, N. ^{[13
]}

Blake, R. S. ^{[1
]}

Carslaw, K. ^{[14
]}

Cooper, O. R. ^{[3
,4
]}

Dentener, F. ^{[15
]}

Fowler, D. ^{[16
]}

Fragkou, E. ^{[17
]}

Frost, G. J. ^{[3
,4
]}

Generoso, S. ^{[18
]}

Ginoux, P. ^{[19
]}

Grewe, V. ^{[20
]}

Guenther, A. ^{[21
]}

Hansson, H. C. ^{[22
]}

Henne, S. ^{[23
]}

Hjorth, J. ^{[15
]}

Hofzumahaus, A. ^{[24
]}

Huntrieser, H. ^{[20
]}

Isaksen, I. S. A. ^{[25
,26
]}

Jenkin, M. E. ^{[27
]}

Kaiser, J. ^{[28
]}

Kanakidou, M. ^{[29
]}

Klimont, Z. ^{[9
]}

Kulmala, M. ^{[30
]}

Laj, P. ^{[31
,32
]}

Lawrence, M. G. ^{[33
]}

Lee, J. D. ^{[34
]}

Liousse, C. ^{[35
]}

Maione, M. ^{[36
]}

McFiggans, G. ^{[37
]}

Metzger, A. ^{[38
]}

Mieville, A. ^{[2
]}

Moussiopoulos, N. ^{[17
]}

Orlando, J. J. ^{[21
]}

O'Dowd, C. D. ^{[39
,40
]}

Palmer, P. I. ^{[41
]}

Parrish, D. D. ^{[3
]}

Petzold, A. ^{[20
]}

Platt, U. ^{[42
]}

Poeschl, U. ^{[33
]}

Prevot, A. S. H. ^{[11
]}

机构：

[1] Univ Leicester, Dept Chem, Leicester LE1 7RH, Leics, England

[2] Univ Paris 06, CNRS INSU, LATMOS IPSL, F-75005 Paris, France

[3] NOAA, Earth Syst Res Lab, Boulder, CO 80305 USA

[4] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA

[5] CNR, Ist Sci Atmosfera & Clima, I-40129 Bologna, Italy

[6] Norwegian Inst Air Res, N-2027 Kjeller, Norway

[7] DEFRA, Air Qual & Ind Pollut Programme, London SW1P 2AL, England

[8] JAMSTEC, Frontier Res Syst Global Change, Yokohama, Kanagawa 2360001, Japan

[9] IIASA, A-2361 Laxenburg, Austria

[10] Danish Meteorol Inst, DK-2100 Copenhagen, Denmark

[11] Paul Scherrer Inst, Lab Atmospher Chem, CH-5232 Villigen, Switzerland

[12] ETH, CH-8092 Zurich, Switzerland

[13] Univ Calif Irvine, Irvine, CA 92697 USA

[14] Univ Leeds, Sch Earth & Environm Sci, Leeds LS2 9JT, W Yorkshire, England

[15] European Commiss, Joint Res Ctr, Inst Environm & Sustainabil, I-21020 Ispra, Italy

[16] Ctr Ecol & Hydrol, Penicuik EH26 0QB, Midlothian, Scotland

[17] Aristotle Univ Thessaloniki, Thessaloniki 54124, Greece

[18] Ecole Polytech Fed Lausanne, LMCA, CH-1015 Lausanne, Switzerland

[19] Princeton Univ, Geophys Fluid Dynam Lab, Princeton, NJ 08540 USA

[20] DLR Inst Phys Atmosphare, D-82230 Wessling, Germany

[21] Natl Ctr Atmospher Res, Boulder, CO 80307 USA

[22] Stockholm Univ, Atmospher Sci Unit, Dept Appl Environm Sci, S-10691 Stockholm, Sweden

[23] Swiss Fed Labs Mat Testing & Res, CH-8600 Dubendorf, Switzerland

[24] KFA Julich GmbH, Forschungszentrum, Inst Chem & Dynam Geosphare, ICG Troposphere 2, D-52425 Julich, Germany

[25] Univ Oslo, Dept Geosci, N-0316 Oslo, Norway

[26] CICERO, N-0318 Oslo, Norway

[27] Atmospher Chem Serv, Okehampton EX20 1FB, England

[28] Univ E Anglia, Sch Environm Sci, Norwich NR4 7TJ, Norfolk, England

[29] Univ Crete, Dept Chem, Iraklion 71003, Greece

[30] Univ Helsinki, Dept Phys, FIN-00014 Helsinki, Finland

[31] Univ Blaise Pascal, CNRS, Lab Meteorol Phys, Observ Phys Globe Clermont Ferrand, F-63177 Clermont Ferrand, France

[32] Univ Grenoble 1, CNRS, Lab Glaciol & Geophys Environm, F-38400 St Martin Dheres, France

[33] Max Planck Inst Chem, D-55128 Mainz, Germany

[34] Univ York, Sch Chem, York YO10 5DD, N Yorkshire, England

[35] Univ Toulouse 3, UMR 5560, Lab Aerol, F-31400 Toulouse, France

[36] Univ Urbino, Ist Sci Chim F Bruner, I-61029 Urbino, Italy

[37] Univ Manchester, Sch Earth Atmospher & Environm Sci, Manchester M13 9PL, Lancs, England

[38] Ionicon Analyt Ges mbH, A-6020 Innsbruck, Austria

[39] Natl Univ Ireland, Sch Phys, Galway, Ireland

[40] Natl Univ Ireland, Ctr Climate & Air Pollut Studies, Environm Change Inst, Galway, Ireland

[41] Univ Edinburgh, Sch Geosci, Edinburgh EH9 3JN, Midlothian, Scotland

[42] Heidelberg Univ, D-69120 Heidelberg, Germany

[43] Weizmann Inst Sci, Dept Environm Sci & Energy Res, IL-76100 Rehovot, Israel

[44] Forschungszentrum Karlsruhe, Inst Meteorol & Climate Res Atmospher Environm Re, D-82467 Garmisch Partenkirchen, Germany

[45] Norwegian Meteorol Inst, EMEP MSC W, N-0313 Oslo, Norway

[46] Chalmers Univ Technol, Dept Radio & Space Sci, S-41296 Gothenburg, Sweden

[47] Energy Res Ctr Netherlands ECN, NL-1755 LE Petten, Netherlands

[48] Univ Stuttgart, D-70049 Stuttgart, Germany

[49] Vrije Univ Amsterdam, NL-1081 HV Amsterdam, Netherlands

[50] CEA, UVSQ, CNRS, Lab Sci Climat & Environm,IPSI, F-91190 Gif Sur Yvette, France

来源：

ATMOSPHERIC ENVIRONMENT | 2009年 / 43卷 / 33期

基金：

美国国家科学基金会;

关键词：

Atmosphere; Troposphere; Air quality; Emissions; Climate; Co-benefit; Oxidation chemistry; Aerosols; Transport of pollutants; Ozone; SECONDARY ORGANIC AEROSOL; MARINE BOUNDARY-LAYER; LONG-RANGE TRANSPORT; TROPOSPHERIC CHEMISTRY MECHANISM; GAS-PHASE OZONOLYSIS; 2003; HEAT-WAVE; VEGETATION ENCLOSURE TECHNIQUES; AIRBORNE PARTICULATE MATTER; RADICAL-INITIATED REACTION; MASTER CHEMICAL MECHANISM;

D O I：

10.1016/j.atmosenv.2009.08.021

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

Air quality transcends all scales with in the atmosphere from the local to the global with handovers and feedbacks at each scale interaction. Air quality has manifold effects on health, ecosystems heritage and, climate. In this review the state of scientific understanding in relation to global and regional air quality is outlined. The review discusses air quality, in terms of emissions, processing and transport of trace gases and aerosols. New insights into the characterization of both natural and anthropogenic emissions are reviewed looking at both natural (e.g. dust and lightning) as well as plant emissions. Trends in anthropogenic emissions both by region and globally are discussed as well as biomass burning emissions. In terms of chemical processing the major air quality elements of ozone, non-methane hydrocarbons, nitrogen oxides and aerosols are covered. A number of topics are presented as a way of integrating the process view into the atmospheric context; these include the atmospheric oxidation efficiency, halogen and HOx chemistry, nighttime chemistry, tropical chemistry, heat waves, megacities, biomass burning and the regional hot spot of the Mediterranean. New findings with respect to the transport of pollutants across the scales are discussed, in particular the move to quantify the impact of long-range transport on regional air quality. Gaps and research questions that remain intractable are identified. The review concludes with a focus of research and policy questions for the coming decade. In particular, the policy challenges for concerted air quality and climate change policy (co-benefit) are discussed. (C) 2009 Elsevier Ltd. All rights reserved.

引用

页码：5268 / 5350

页数：83

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